| 1 | I Can't Help Myself (Sugar Pie Honey Bunch)Four Tops | 4 | Chart history → |
| 2 | Mr. Tambourine ManThe Byrds | 6 | Chart history → |
| 3 | Wooly BullySam The Sham and the Pharaohs | 2 | Chart history → |
| 4 | Crying In The ChapelElvis Presley With The Jordanaires | 3 | Chart history → |
| 5 | Back In My Arms AgainThe Supremes | 1 | Chart history → |
| 6 | Wonderful WorldHerman's Hermits | 8 | Chart history → |
| 7 | Help Me, RhondaThe Beach Boys | 5 | Chart history → |
| 8 | Engine Engine #9Roger Miller | 7 | Chart history → |
| 9 | For Your LoveThe Yardbirds | 13 | Chart history → |
| 10 | Hush, Hush, Sweet CharlottePatti Page | 14 | Chart history → |
| 11 | Ticket To RideThe Beatles | 9 | Chart history → |
| 12 | Just A LittleThe Beau Brummels | 10 | Chart history → |
| 13 | Last Chance To Turn AroundGene Pitney | 16 | Chart history → |
| 14 | Mrs. Brown You've Got A Lovely DaughterHerman's Hermits | 11 | Chart history → |
| 15 | Seventh SonJohnny Rivers | 43 | Chart history → |
| 16 | A Walk In The Black ForestHorst Jankowski | 29 | Chart history → |
| 17 | Before And AfterChad & Jeremy | 25 | Chart history → |
| 18 | Nothing Can Stop MeGene Chandler | 24 | Chart history → |
| 19 | True Love WaysPeter And Gordon | 19 | Chart history → |
| 20 | It's Not UnusualTom Jones | 12 | Chart history → |
| 21 | You Turn Me On (Turn On Song)Ian Whitcomb And Bluesville | 51 | Chart history → |
| 22 | What The World Needs Now Is LoveJackie DeShannon | 41 | Chart history → |
| 23 | Yes, I'm ReadyBarbara Mason | 40 | Chart history → |
| 24 | Shakin' All OverThe Guess Who | 27 | Chart history → |
| 25 | Catch The WindDonovan | 31 | Chart history → |
| 26 | (I Can't Get No) SatisfactionThe Rolling Stones | 67 | Chart history → |
| 27 | L-O-N-E-L-YBobby Vinton | 22 | Chart history → |
| 28 | Cara, MiaJay & The Americans | 54 | Chart history → |
| 29 | Laurie (Strange Things Happen)Dickey Lee | 47 | Chart history → |
| 30 | Voodoo WomanBobby Goldsboro | 37 | Chart history → |
| 31 | SilhouettesHerman's Hermits | 18 | Chart history → |
| 32 | (Remember Me) I'm The One Who Loves YouDean Martin | 34 | Chart history → |
| 33 | Just Once In My LifeThe Righteous Brothers | 21 | Chart history → |
| 34 | You Were Only Fooling (While I Was Falling In Love)Vic Damone | 30 | Chart history → |
| 35 | Give Us Your BlessingsThe Shangri-Las | 42 | Chart history → |
| 36 | I've Been Loving You Too Long (To Stop Now)Otis Redding | 46 | Chart history → |
| 37 | Concrete And ClayUnit Four plus Two | 28 | Chart history → |
| 38 | Oo Wee Baby, I Love YouFred Hughes | 45 | Chart history → |
| 39 | Cast Your Fate To The WindSounds Orchestral | 36 | Chart history → |
| 40 | Bring It On Home To MeThe Animals | 32 | Chart history → |
| 41 | You Really Know How To Hurt A GuyJan & Dean | 44 | Chart history → |
| 42 | Three O'Clock In The MorningBert Kaempfert And His Orchestra | 33 | Chart history → |
| 43 | Queen Of The HouseJody Miller | 20 | Chart history → |
| 44 | A World Of Our OwnThe Seekers | 57 | Chart history → |
| 45 | Here Comes The NightThem | 53 | Chart history → |
| 46 | Concrete And ClayEddie Rambeau | 35 | Chart history → |
| 47 | A Little Bit Of HeavenRonnie Dove | 68 | Chart history → |
| 48 | I DoThe Marvelows | 58 | Chart history → |
| 49 | This Little BirdMarianne Faithfull | 59 | Chart history → |
| 50 | I'll Never Find Another YouThe Seekers | 17 | Chart history → |
| 51 | I'll Keep Holding OnThe Marvelettes | 61 | Chart history → |
| 52 | I'll Be With You In Apple Blossom TimeWayne Newton | 52 | Chart history → |
| 53 | Too Many RiversBrenda Lee | 63 | Chart history → |
| 54 | Tonight's The NightSolomon Burke | 70 | Chart history → |
| 55 | And I Love HimEsther Phillips | 56 | Chart history → |
| 56 | She's About A MoverSir Douglas Quintet | 15 | Chart history → |
| 57 | Lipstick Traces (On A Cigarette)The O'Jays | 48 | Chart history → |
| 58 | Little Lonely OneTom Jones | 60 | Chart history → |
| 59 | Something You GotChuck Jackson & Maxine Brown | 55 | Chart history → |
| 60 | Do The BoomerangJr. Walker & The All Stars | 72 | Chart history → |
| 61 | It's Wonderful To Be In LoveThe Ovations (Featuring Louis Williams) | 66 | Chart history → |
| 62 | When A Boy Falls In LoveSam Cooke | 74 | Chart history → |
| 63 | You'll Never Walk AloneGerry And The Pacemakers | 76 | Chart history → |
| 64 | Tell Her (You Love Her Every Day)Frank Sinatra | 64 | Chart history → |
| 65 | Boo-Ga-LooTom and Jerrio | 62 | Chart history → |
| 66 | Love Is A 5-Letter WordJames Phelps | 71 | Chart history → |
| 67 | Bring A Little Sunshine (To My Heart)Vic Dana | 69 | Chart history → |
| 68 | Set Me FreeThe Kinks | 83 | Chart history → |
| 69 | What's He Doing In My WorldEddy Arnold | 73 | Chart history → |
| 70 | (Such An) Easy QuestionElvis Presley With The Jordanaires | — | Chart history → |
| 71 | MarieThe Bachelors | 89 | Chart history → |
| 72 | Who's Cheating Who?Little Milton | 84 | Chart history → |
| 73 | Meeting Over YonderThe Impressions | 79 | Chart history → |
| 74 | I Love You SoBobbi Martin | 77 | Chart history → |
| 75 | Is This What I Get For Loving You?The Ronettes Featuring Veronica | 75 | Chart history → |
| 76 | Summer SoundsRobert Goulet | 78 | Chart history → |
| 77 | Temptation 'Bout To Get MeThe Knight Bros. | 82 | Chart history → |
| 78 | The Puzzle Song (A Puzzle In Song)Shirley Ellis | 80 | Chart history → |
| 79 | What's New Pussycat?Tom Jones | — | Chart history → |
| 80 | It's Just A Little Bit Too LateWayne Fontana & The Mindbenders | 88 | Chart history → |
| 81 | It Feels So RightElvis Presley With The Jordanaires | — | Chart history → |
| 82 | Girl Come RunningThe 4 Seasons Featuring the "Sound of Frankie Valli" | — | Chart history → |
| 83 | I Like It Like ThatThe Dave Clark Five | — | Chart history → |
| 84 | Lip Sync (To The Tongue Twisters)Len Barry | 86 | Chart history → |
| 85 | Boot-LegBooker T. & The MG's | 85 | Chart history → |
| 86 | Seein' The Right Love Go WrongJack Jones | 95 | Chart history → |
| 87 | OperatorBrenda Holloway | 87 | Chart history → |
| 88 | Then I'll Count AgainJohnny Tillotson | 92 | Chart history → |
| 89 | My CherieAl Martino | 90 | Chart history → |
| 90 | He's A LoverMary Wells | — | Chart history → |
| 91 | Ain't It A ShameMajor Lance | 91 | Chart history → |
| 92 | Sitting In The ParkBilly Stewart | — | Chart history → |
| 93 | From The Bottom Of My Heart (I Love You)The Moody Blues | 97 | Chart history → |
| 94 | Soul Sauce (Guacha Guaro)Cal Tjader | 94 | Chart history → |
| 95 | Welcome HomeWalter Jackson | 99 | Chart history → |
| 96 | Are You SincereTrini Lopez | 98 | Chart history → |
| 97 | Baby, I'm YoursBarbara Lewis | — | Chart history → |
| 98 | Sunshine, Lollipops And RainbowsLesley Gore | — | Chart history → |
| 99 | Long Live LoveSandie Shaw | 100 | Chart history → |
| 100 | Nobody Knows What's Goin' On (In My Mind But Me)The Chiffons | — | Chart history → |