| 1 | Reach Out I'll Be ThereFour Tops | 1 | Chart history → |
| 2 | 96 Tears? (Question Mark) & The Mysterians | 3 | Chart history → |
| 3 | Last Train To ClarksvilleThe Monkees | 4 | Chart history → |
| 4 | CherishThe Association | 2 | Chart history → |
| 5 | Psychotic ReactionCount Five | 5 | Chart history → |
| 6 | Walk Away ReneeThe Left Banke | 7 | Chart history → |
| 7 | Poor Side Of TownJohnny Rivers | 11 | Chart history → |
| 8 | What Becomes Of The BrokenheartedJimmy Ruffin | 8 | Chart history → |
| 9 | DandyHerman's Hermits | 15 | Chart history → |
| 10 | See See RiderEric Burdon & The Animals | 14 | Chart history → |
| 11 | Hooray For HazelTommy Roe | 16 | Chart history → |
| 12 | If I Were A CarpenterBobby Darin | 17 | Chart history → |
| 13 | Have You Seen Your Mother, Baby, Standing In The Shadow?The Rolling Stones | 18 | Chart history → |
| 14 | Cherry, CherryNeil Diamond | 6 | Chart history → |
| 15 | I've Got You Under My SkinThe 4 Seasons Featuring the "Sound of Frankie Valli" | 9 | Chart history → |
| 16 | B-A-B-YCarla Thomas | 19 | Chart history → |
| 17 | Go Away Little GirlThe Happenings | 42 | Chart history → |
| 18 | You Can't Hurry LoveThe Supremes | 10 | Chart history → |
| 19 | Black Is BlackLos Bravos | 13 | Chart history → |
| 20 | All I See Is YouDusty Springfield | 21 | Chart history → |
| 21 | The Great Airplane StrikePaul Revere & The Raiders Featuring Mark Lindsay | 35 | Chart history → |
| 22 | Beauty Is Only Skin DeepThe Temptations | 12 | Chart history → |
| 23 | Little ManSonny & Cher | 28 | Chart history → |
| 24 | Love Is A Hurtin' ThingLou Rawls | 38 | Chart history → |
| 25 | Born FreeRoger Williams | 31 | Chart history → |
| 26 | All Strung OutNino Tempo & April Stevens | 27 | Chart history → |
| 27 | The Hair On My Chinny Chin ChinSam The Sham and the Pharaohs | 36 | Chart history → |
| 28 | Girl On A SwingGerry And The Pacemakers | 30 | Chart history → |
| 29 | I Really Don't Want To KnowRonnie Dove | 22 | Chart history → |
| 30 | Wipe OutThe Surfaris | 25 | Listen & explore → |
| 31 | Born A WomanSandy Posey | 24 | Chart history → |
| 32 | I Can Make It With YouPozo Seco Singers | 34 | Chart history → |
| 33 | I'm Your PuppetJames & Bobby Purify | 49 | Chart history → |
| 34 | Devil With A Blue Dress On & Good Golly Miss MollyMitch Ryder And The Detroit Wheels | 59 | Chart history → |
| 35 | I Just Don't Know What To Do With MyselfDionne Warwick | 45 | Chart history → |
| 36 | Mr. Dieingly SadThe Critters | 20 | Chart history → |
| 37 | (You Don't Have To) Paint Me A PictureGary Lewis And The Playboys | 50 | Chart history → |
| 38 | Mr. SpacemanThe Byrds | 43 | Chart history → |
| 39 | Summer Samba (So Nice)Walter Wanderley | 26 | Chart history → |
| 40 | Rain On The RoofThe Lovin' Spoonful | 76 | Chart history → |
| 41 | Bus StopThe Hollies | 23 | Chart history → |
| 42 | Coming On StrongBrenda Lee | 53 | Chart history → |
| 43 | Almost PersuadedDavid Houston | 33 | Chart history → |
| 44 | Come On UpThe Young Rascals | 44 | Chart history → |
| 45 | Fa-Fa-Fa-Fa-Fa (Sad Song)Otis Redding | 55 | Chart history → |
| 46 | I Want To Be With YouDee Dee Warwick | 47 | Chart history → |
| 47 | SpinoutElvis Presley With The Jordanaires | 57 | Chart history → |
| 48 | Please Mr. SunThe Vogues | 58 | Chart history → |
| 49 | Mas Que NadaSergio Mendes & Brasil '66 | 51 | Chart history → |
| 50 | Sunshine SupermanDonovan | 29 | Chart history → |
| 51 | Mind ExcursionThe Trade Winds | 52 | Chart history → |
| 52 | All That I AmElvis Presley With The Jordanaires | 62 | Chart history → |
| 53 | In Our TimeNancy Sinatra | 46 | Chart history → |
| 54 | Ain't Gonna LieKeith | 66 | Chart history → |
| 55 | A Satisfied MindBobby Hebb | 67 | Chart history → |
| 56 | But It's AlrightJ.J. Jackson | 68 | Chart history → |
| 57 | Lady GodivaPeter And Gordon | 75 | Chart history → |
| 58 | Up TightRamsey Lewis | 74 | Chart history → |
| 59 | Secret LoveBilly Stewart | 73 | Chart history → |
| 60 | Almost Persuaded No. 2Ben Colder | 60 | Chart history → |
| 61 | The Fife PiperThe Dynatones | 56 | Chart history → |
| 62 | Knock On WoodEddie Floyd | 72 | Chart history → |
| 63 | ChangesCrispian St. Peters | 64 | Chart history → |
| 64 | Baby, Do The Philly DogThe Olympics | 86 | Chart history → |
| 65 | Look Through My WindowThe Mamas & The Papas | — | Chart history → |
| 66 | I Can't Control MyselfThe Troggs | 85 | Chart history → |
| 67 | Don't Worry Mother, Your Son's Heart Is PureThe McCoys | 70 | Chart history → |
| 68 | The Wheel Of HurtMargaret Whiting | 79 | Chart history → |
| 69 | Don't Be A Drop-OutJames Brown And The Famous Flames | 82 | Chart history → |
| 70 | Who Am IPetula Clark | — | Chart history → |
| 71 | I've Got To Do A Little Bit BetterJoe Tex | 81 | Chart history → |
| 72 | Nobody's Baby AgainDean Martin | 87 | Chart history → |
| 73 | Stay With MeLorraine Ellison | 92 | Chart history → |
| 74 | Louie, LouieThe Sandpipers | — | Chart history → |
| 75 | Somebody (Somewhere) Needs YouDarrell Banks | 83 | Chart history → |
| 76 | Somebody Like MeEddy Arnold | 88 | Chart history → |
| 77 | The Wheel Of HurtAl Martino | 99 | Chart history → |
| 78 | HappinessShades Of Blue | 78 | Chart history → |
| 79 | Take Good Care Of HerMel Carter | 84 | Chart history → |
| 80 | Tomorrow Never ComesB.J. Thomas | 80 | Chart history → |
| 81 | Good VibrationsThe Beach Boys | — | Chart history → |
| 82 | Heaven Must Have Sent YouThe Elgins | — | Chart history → |
| 83 | Wish You Were Here, BuddyPat Boone | — | Chart history → |
| 84 | Nineteen DaysThe Dave Clark Five | — | Chart history → |
| 85 | Holy CowLee Dorsey | — | Chart history → |
| 86 | A Symphony For SusanThe Arbors | 95 | Chart history → |
| 87 | Whispers (Gettin' Louder)Jackie Wilson | 90 | Chart history → |
| 88 | Free AgainBarbra Streisand | 89 | Chart history → |
| 89 | You Are SheChad & Jeremy | 91 | Chart history → |
| 90 | Run, Run, Look And SeeBrian Hyland | — | Chart history → |
| 91 | Pouring Water On A Drowning ManJames Carr | — | Chart history → |
| 92 | It Tears Me UpPercy Sledge | — | Chart history → |
| 93 | Why Pick On MeThe Standells | — | Chart history → |
| 94 | Bang BangThe Joe Cuba Sextet | — | Chart history → |
| 95 | Cry SoftlyNancy Ames | 98 | Chart history → |
| 96 | Every Day And Every NightThe Trolls | — | Chart history → |
| 97 | PovertyBobby Bland | — | Chart history → |
| 98 | Stand In For LoveThe O'Jays | — | Chart history → |
| 99 | Don't Answer The Door - Part 1B.B. King | — | Chart history → |
| 100 | Games That Lovers PlayWayne Newton | — | Chart history → |