| 1 | Last Train To ClarksvilleThe Monkees | 2 | Chart history → |
| 2 | 96 Tears? (Question Mark) & The Mysterians | 1 | Chart history → |
| 3 | Poor Side Of TownJohnny Rivers | 4 | Chart history → |
| 4 | Reach Out I'll Be ThereFour Tops | 3 | Chart history → |
| 5 | DandyHerman's Hermits | 6 | Chart history → |
| 6 | Hooray For HazelTommy Roe | 8 | Chart history → |
| 7 | What Becomes Of The BrokenheartedJimmy Ruffin | 7 | Chart history → |
| 8 | If I Were A CarpenterBobby Darin | 11 | Chart history → |
| 9 | Have You Seen Your Mother, Baby, Standing In The Shadow?The Rolling Stones | 9 | Chart history → |
| 10 | Walk Away ReneeThe Left Banke | 5 | Chart history → |
| 11 | I'm Your PuppetJames & Bobby Purify | 16 | Chart history → |
| 12 | Go Away Little GirlThe Happenings | 12 | Chart history → |
| 13 | Love Is A Hurtin' ThingLou Rawls | 19 | Chart history → |
| 14 | B-A-B-YCarla Thomas | 15 | Chart history → |
| 15 | (You Don't Have To) Paint Me A PictureGary Lewis And The Playboys | 18 | Chart history → |
| 16 | See See RiderEric Burdon & The Animals | 10 | Chart history → |
| 17 | Good VibrationsThe Beach Boys | 38 | Chart history → |
| 18 | Devil With A Blue Dress On & Good Golly Miss MollyMitch Ryder And The Detroit Wheels | 27 | Chart history → |
| 19 | Born FreeRoger Williams | 24 | Chart history → |
| 20 | Rain On The RoofThe Lovin' Spoonful | 26 | Chart history → |
| 21 | CherishThe Association | 13 | Chart history → |
| 22 | The Hair On My Chinny Chin ChinSam The Sham and the Pharaohs | 22 | Chart history → |
| 23 | Psychotic ReactionCount Five | 14 | Chart history → |
| 24 | Winchester CathedralThe New Vaudeville Band | 66 | Chart history → |
| 25 | Coming On StrongBrenda Lee | 31 | Chart history → |
| 26 | The Great Airplane StrikePaul Revere & The Raiders Featuring Mark Lindsay | 20 | Chart history → |
| 27 | You Keep Me Hangin' OnThe Supremes | 68 | Chart history → |
| 28 | I Just Don't Know What To Do With MyselfDionne Warwick | 30 | Chart history → |
| 29 | Lady GodivaPeter And Gordon | 46 | Chart history → |
| 30 | Who Am IPetula Clark | 39 | Chart history → |
| 31 | Cherry, CherryNeil Diamond | 17 | Chart history → |
| 32 | Fa-Fa-Fa-Fa-Fa (Sad Song)Otis Redding | 34 | Chart history → |
| 33 | I Can Make It With YouPozo Seco Singers | 33 | Chart history → |
| 34 | Look Through My WindowThe Mamas & The Papas | 51 | Chart history → |
| 35 | Little ManSonny & Cher | 21 | Chart history → |
| 36 | I've Got You Under My SkinThe 4 Seasons Featuring the "Sound of Frankie Valli" | 23 | Chart history → |
| 37 | Secret LoveBilly Stewart | 49 | Chart history → |
| 38 | But It's AlrightJ.J. Jackson | 54 | Chart history → |
| 39 | A Satisfied MindBobby Hebb | 45 | Chart history → |
| 40 | SpinoutElvis Presley With The Jordanaires | 44 | Chart history → |
| 41 | Ain't Gonna LieKeith | 52 | Chart history → |
| 42 | All That I AmElvis Presley With The Jordanaires | 42 | Chart history → |
| 43 | Stop Stop StopThe Hollies | 76 | Chart history → |
| 44 | Girl On A SwingGerry And The Pacemakers | 32 | Chart history → |
| 45 | I Can't Control MyselfThe Troggs | 55 | Chart history → |
| 46 | Louie, LouieThe Sandpipers | 59 | Chart history → |
| 47 | Mas Que NadaSergio Mendes & Brasil '66 | 47 | Chart history → |
| 48 | Beauty Is Only Skin DeepThe Temptations | 37 | Chart history → |
| 49 | Up TightRamsey Lewis | 50 | Chart history → |
| 50 | You Can't Hurry LoveThe Supremes | 25 | Chart history → |
| 51 | Come On UpThe Young Rascals | 43 | Chart history → |
| 52 | Please Mr. SunThe Vogues | 48 | Chart history → |
| 53 | Don't Be A Drop-OutJames Brown And The Famous Flames | 56 | Chart history → |
| 54 | All I See Is YouDusty Springfield | 29 | Chart history → |
| 55 | Mr. SpacemanThe Byrds | 36 | Chart history → |
| 56 | The Wheel Of HurtMargaret Whiting | 67 | Chart history → |
| 57 | I'm Ready For LoveMartha & The Vandellas | 70 | Chart history → |
| 58 | Knock On WoodEddie Floyd | 62 | Chart history → |
| 59 | Nineteen DaysThe Dave Clark Five | 69 | Chart history → |
| 60 | Nobody's Baby AgainDean Martin | 60 | Chart history → |
| 61 | Somebody Like MeEddy Arnold | 61 | Chart history → |
| 62 | It Tears Me UpPercy Sledge | 79 | Chart history → |
| 63 | I Want To Be With YouDee Dee Warwick | 41 | Chart history → |
| 64 | Heaven Must Have Sent YouThe Elgins | 72 | Chart history → |
| 65 | Holy CowLee Dorsey | 82 | Chart history → |
| 66 | Almost Persuaded No. 2Ben Colder | 58 | Chart history → |
| 67 | I've Got To Do A Little Bit BetterJoe Tex | 64 | Chart history → |
| 68 | On This Side Of GoodbyeThe Righteous Brothers | 77 | Chart history → |
| 69 | Mind ExcursionThe Trade Winds | 65 | Chart history → |
| 70 | Baby, Do The Philly DogThe Olympics | 63 | Chart history → |
| 71 | Stay With MeLorraine Ellison | 71 | Chart history → |
| 72 | Why Pick On MeThe Standells | 89 | Chart history → |
| 73 | The Wheel Of HurtAl Martino | 74 | Chart history → |
| 74 | Somebody (Somewhere) Needs YouDarrell Banks | 75 | Chart history → |
| 75 | Bang BangThe Joe Cuba Sextet | 88 | Chart history → |
| 76 | Wish You Were Here, BuddyPat Boone | 81 | Chart history → |
| 77 | Run, Run, Look And SeeBrian Hyland | 83 | Chart history → |
| 78 | Whispers (Gettin' Louder)Jackie Wilson | — | Chart history → |
| 79 | Baby What Do You Want Me To DoBarbara Lewis | 86 | Chart history → |
| 80 | A Symphony For SusanThe Arbors | 80 | Chart history → |
| 81 | A Hazy Shade Of WinterSimon & Garfunkel | — | Chart history → |
| 82 | (When She Needs Good Lovin') She Comes To MeThe Chicago Loop | — | Chart history → |
| 83 | Free AgainBarbra Streisand | 84 | Chart history → |
| 84 | A Day In The Life Of A FoolJack Jones | 85 | Chart history → |
| 85 | Time After TimeChris Montez | 93 | Chart history → |
| 86 | Come BackThe Five Stairsteps | — | Chart history → |
| 87 | Don't Answer The Door - Part 1B.B. King | 98 | Chart history → |
| 88 | Help Me GirlThe Outsiders | 90 | Chart history → |
| 89 | Pouring Water On A Drowning ManJames Carr | 91 | Chart history → |
| 90 | (Come 'round Here) I'm The One You NeedThe Miracles | — | Chart history → |
| 91 | Games That Lovers PlayEddie Fisher | 92 | Chart history → |
| 92 | Heartbreak HotelRoger Miller | — | Chart history → |
| 93 | Games That Lovers PlayWayne Newton | 94 | Chart history → |
| 94 | A Corner In The SunWalter Jackson | — | Chart history → |
| 95 | Stand In For LoveThe O'Jays | 96 | Chart history → |
| 96 | It's Only LoveTommy James And The Shondells | — | Chart history → |
| 97 | Can I Get To Know You BetterThe Turtles | 99 | Chart history → |
| 98 | Winchester CathedralDana Rollin | — | Chart history → |
| 99 | Spanish Nights And YouConnie Francis | — | Chart history → |
| 100 | Meditation (Meditacao)Claudine Longet | — | Chart history → |