| 1 | Winchester CathedralThe New Vaudeville Band | 1 | Chart history → |
| 2 | Mellow YellowDonovan | 2 | Chart history → |
| 3 | I'm A BelieverThe Monkees | 8 | Chart history → |
| 4 | That's LifeFrank Sinatra | 6 | Chart history → |
| 5 | Devil With A Blue Dress On & Good Golly Miss MollyMitch Ryder And The Detroit Wheels | 4 | Chart history → |
| 6 | Sugar TownNancy Sinatra | 9 | Chart history → |
| 7 | Snoopy Vs. The Red BaronThe Royal Guardsmen | 30 | Chart history → |
| 8 | Good VibrationsThe Beach Boys | 3 | Chart history → |
| 9 | A Place In The SunStevie Wonder | 10 | Chart history → |
| 10 | (I Know) I'm Losing YouThe Temptations | 12 | Chart history → |
| 11 | You Keep Me Hangin' OnThe Supremes | 5 | Chart history → |
| 12 | Born FreeRoger Williams | 7 | Chart history → |
| 13 | Whispers (Gettin' Louder)Jackie Wilson | 11 | Chart history → |
| 14 | Tell It Like It IsAaron Neville | 25 | Chart history → |
| 15 | Lady GodivaPeter And Gordon | 13 | Chart history → |
| 16 | I Got The Feelin' (Oh No No)Neil Diamond | 16 | Chart history → |
| 17 | Single GirlSandy Posey | 23 | Chart history → |
| 18 | CryRonnie Dove | 26 | Chart history → |
| 19 | MameHerb Alpert & The Tijuana Brass | 19 | Chart history → |
| 20 | Coming Home SoldierBobby Vinton | 32 | Chart history → |
| 21 | Talk TalkThe Music Machine | 24 | Chart history → |
| 22 | I Need Somebody? (Question Mark) & The Mysterians | 27 | Chart history → |
| 23 | Mustang SallyWilson Pickett | 29 | Chart history → |
| 24 | Words Of LoveThe Mamas & The Papas | 36 | Chart history → |
| 25 | I'm Ready For LoveMartha & The Vandellas | 14 | Chart history → |
| 26 | Stop Stop StopThe Hollies | 18 | Chart history → |
| 27 | Good ThingPaul Revere & The Raiders Featuring Mark Lindsay | 35 | Chart history → |
| 28 | A Hazy Shade Of WinterSimon & Garfunkel | 15 | Chart history → |
| 29 | East WestHerman's Hermits | 41 | Chart history → |
| 30 | (Come 'round Here) I'm The One You NeedThe Miracles | 17 | Chart history → |
| 31 | Tell It To The RainThe 4 Seasons Featuring the "Sound of Frankie Valli" | 58 | Chart history → |
| 32 | It's Only LoveTommy James And The Shondells | 31 | Chart history → |
| 33 | I've Passed This Way BeforeJimmy Ruffin | 46 | Chart history → |
| 34 | Knock On WoodEddie Floyd | 28 | Chart history → |
| 35 | Pandora's Golden Heebie JeebiesThe Association | 39 | Chart history → |
| 36 | I'm Your PuppetJames & Bobby Purify | 21 | Chart history → |
| 37 | It Tears Me UpPercy Sledge | 20 | Chart history → |
| 38 | Standing In The Shadows Of LoveFour Tops | 62 | Chart history → |
| 39 | Poor Side Of TownJohnny Rivers | 22 | Chart history → |
| 40 | Happenings Ten Years Time AgoThe Yardbirds | 47 | Chart history → |
| 41 | Help Me GirlEric Burdon & The Animals | 49 | Chart history → |
| 42 | But It's AlrightJ.J. Jackson | 34 | Chart history → |
| 43 | Help Me GirlThe Outsiders | 37 | Chart history → |
| 44 | Coming On StrongBrenda Lee | 33 | Chart history → |
| 45 | Nashville CatsThe Lovin' Spoonful | 86 | Chart history → |
| 46 | Try A Little TendernessOtis Redding | 56 | Chart history → |
| 47 | Games That Lovers PlayEddie Fisher | 45 | Chart history → |
| 48 | (I'm Not Your) Steppin' StoneThe Monkees | 77 | Chart history → |
| 49 | I Fooled You This TimeGene Chandler | 48 | Chart history → |
| 50 | Georgy GirlThe Seekers | 59 | Chart history → |
| 51 | I (Who Have Nothing)Terry Knight and The Pack | 51 | Chart history → |
| 52 | Ghost Riders In The SkyBaja Marimba Band | 57 | Chart history → |
| 53 | The Eggplant That Ate ChicagoDr. West's Medicine Show and Junk Band | 53 | Chart history → |
| 54 | Blue AutumnBobby Goldsboro | 63 | Chart history → |
| 55 | There's Got To Be A Word!The Innocence | 55 | Chart history → |
| 56 | Goodnight My LoveThe Happenings | 66 | Chart history → |
| 57 | 98.6Keith | 73 | Chart history → |
| 58 | Bad MisunderstandingThe Critters | 64 | Chart history → |
| 59 | Please Don't Ever Leave MeThe Cyrkle | 61 | Chart history → |
| 60 | (We Ain't Got) Nothin' YetBlues Magoos | 74 | Chart history → |
| 61 | Where Will The Words Come FromGary Lewis And The Playboys | 87 | Chart history → |
| 62 | You Can Bring Me All Your HeartachesLou Rawls | 68 | Chart history → |
| 63 | KarateThe Emperor's | 84 | Chart history → |
| 64 | Baby What I MeanThe Drifters | 71 | Chart history → |
| 65 | Gallant MenSenator Everett McKinley Dirksen | — | Chart history → |
| 66 | The Girl That Stood Beside MeBobby Darin | 75 | Chart history → |
| 67 | Money (That's What I Want) (Part 1)Jr. Walker & The All Stars | 52 | Chart history → |
| 68 | I Had Too Much To Dream (Last Night)The Electric Prunes | 81 | Chart history → |
| 69 | Color My WorldPetula Clark | — | Chart history → |
| 70 | Papa Was TooJoe Tex | 83 | Chart history → |
| 71 | (Open Up The Door) Let The Good Times InDean Martin | 93 | Chart history → |
| 72 | Communication BreakdownRoy Orbison | 79 | Chart history → |
| 73 | There's Something On Your MindBaby Ray | 78 | Chart history → |
| 74 | Alvin's Boo-Ga-LooAlvin Cash & The Registers | 76 | Chart history → |
| 75 | Another NightDionne Warwick | — | Chart history → |
| 76 | Green, Green Grass Of HomeTom Jones | — | Chart history → |
| 77 | Dancing In The StreetThe Mamas & The Papas | 94 | Chart history → |
| 78 | How Do You Catch A GirlSam The Sham and the Pharaohs | — | Chart history → |
| 79 | Look What You've DonePozo Seco Singers | 98 | Chart history → |
| 80 | Day TripperRamsey Lewis | — | Chart history → |
| 81 | Wack WackThe Young Holt Trio | 91 | Chart history → |
| 82 | Stand By MeSpyder Turner | 99 | Chart history → |
| 83 | I'm Gonna Miss YouThe Artistics | 88 | Chart history → |
| 84 | If You Go AwayDamita Jo | 89 | Chart history → |
| 85 | Grizzly BearThe Youngbloods | 95 | Chart history → |
| 86 | Knight In Rusty ArmourPeter And Gordon | — | Chart history → |
| 87 | It's Now Winters DayTommy Roe | — | Chart history → |
| 88 | Just One SmileGene Pitney | — | Chart history → |
| 89 | Constant Rain (Chove Chuva)Sergio Mendes & Brasil '66 | — | Chart history → |
| 90 | I'm Gonna Make You MineThe Shadows Of Knight | — | Chart history → |
| 91 | Going NowhereLos Bravos | 96 | Chart history → |
| 92 | Look At Granny Run, RunHoward Tate | — | Chart history → |
| 93 | Are You Lonely For MeFreddy Scott | — | Chart history → |
| 94 | The Shadow Of Your SmileBoots Randolph | — | Chart history → |
| 95 | Pushin' Too HardThe Seeds | — | Chart history → |
| 96 | Wish Me A RainbowThe Gunter Kallmann Chorus | — | Chart history → |
| 97 | Try My Love AgainBobby Moore's Rhythm Aces featuring Chico | 100 | Chart history → |
| 98 | Any Way That You Want MeLiverpool Five | — | Chart history → |
| 99 | That's The TuneThe Vogues | — | Chart history → |
| 100 | Hello HelloThe Sopwith "Camel" | — | Chart history → |