| 1 | Green TambourineThe Lemon Pipers | 3 | Chart history → |
| 2 | Judy In Disguise (With Glasses)John Fred And The Playboys | 1 | Chart history → |
| 3 | Chain Of FoolsAretha Franklin | 2 | Chart history → |
| 4 | SpookyClassics IV | 7 | Chart history → |
| 5 | Bend Me, Shape MeThe American Breed | 5 | Chart history → |
| 6 | Woman, WomanThe Union Gap Featuring Gary Puckett | 4 | Chart history → |
| 7 | Love Is Blue (L'amour Est Bleu)Paul Mauriat And His Orchestra | 18 | Chart history → |
| 8 | Nobody But MeThe Human Beinz | 12 | Chart history → |
| 9 | Goin' Out Of My Head/Can't Take My Eyes Off YouThe Lettermen | 17 | Chart history → |
| 10 | I Wish It Would RainThe Temptations | 15 | Chart history → |
| 11 | SusanThe Buckinghams | 11 | Chart history → |
| 12 | Hello GoodbyeThe Beatles | 6 | Chart history → |
| 13 | Baby, Now That I've Found YouThe Foundations | 20 | Chart history → |
| 14 | Different DrumStone Poneys Featuring Linda Ronstadt | 13 | Chart history → |
| 15 | I Heard It Through The GrapevineGladys Knight And The Pips | 9 | Chart history → |
| 16 | Itchycoo ParkSmall Faces | 16 | Chart history → |
| 17 | I Second That EmotionSmokey Robinson & The Miracles | 14 | Chart history → |
| 18 | Am I That Easy To ForgetEngelbert Humperdinck | 19 | Chart history → |
| 19 | Darlin'The Beach Boys | 24 | Chart history → |
| 20 | I Wonder What She's Doing ToniteTommy Boyce & Bobby Hart | 26 | Chart history → |
| 21 | My Baby Must Be A MagicianThe Marvelettes | 21 | Chart history → |
| 22 | Bottle Of WineThe Fireballs | 28 | Chart history → |
| 23 | Tell MamaEtta James | 23 | Chart history → |
| 24 | Daydream BelieverThe Monkees | 8 | Chart history → |
| 25 | Love PowerThe Sandpebbles | 22 | Chart history → |
| 26 | Skip A RopeHenson Cargill | 35 | Chart history → |
| 27 | Just As Much As EverBobby Vinton | 32 | Chart history → |
| 28 | TomorrowStrawberry Alarm Clock | 29 | Chart history → |
| 29 | If I Could Build My Whole World Around YouMarvin Gaye & Tammi Terrell | 10 | Chart history → |
| 30 | To Give (The Reason I Live)Frankie Valli | 30 | Chart history → |
| 31 | Sunday Mornin'Spanky And Our Gang | 41 | Chart history → |
| 32 | Some Velvet MorningNancy Sinatra & Lee Hazlewood | 39 | Chart history → |
| 33 | (Theme From) Valley Of The DollsDionne Warwick | 61 | Chart history → |
| 34 | We Can FlyThe Cowsills | 44 | Chart history → |
| 35 | YouMarvin Gaye | 45 | Chart history → |
| 36 | We're A WinnerThe Impressions | 47 | Chart history → |
| 37 | She's A RainbowThe Rolling Stones | 25 | Chart history → |
| 38 | I Can Take Or Leave Your LovingHerman's Hermits | 48 | Chart history → |
| 39 | MontereyEric Burdon & The Animals | 37 | Chart history → |
| 40 | Explosion (In Your Soul)Soul Survivors | 33 | Chart history → |
| 41 | Back Up TrainAl Greene & The Soul Mate's | 51 | Chart history → |
| 42 | Skinny Legs And AllJoe Tex | 40 | Chart history → |
| 43 | Two Little KidsPeaches & Herb | 31 | Chart history → |
| 44 | The LessonVikki Carr | 34 | Chart history → |
| 45 | Boogaloo Down BroadwayThe Fantastic Johnny C | 42 | Chart history → |
| 46 | WordsBee Gees | 64 | Chart history → |
| 47 | (Sittin' On) The Dock Of The BayOtis Redding | 67 | Chart history → |
| 48 | MoneyThe Lovin' Spoonful | 49 | Chart history → |
| 49 | No Sad SongsJoe Simon | 50 | Chart history → |
| 50 | Strawberry ShortcakeJay And The Techniques | 60 | Chart history → |
| 51 | New OrleansNeil Diamond | 52 | Chart history → |
| 52 | ZabadakDave Dee, Dozy, Beaky, Mick And Tich | 55 | Chart history → |
| 53 | CarmenHerb Alpert & The Tijuana Brass | 63 | Chart history → |
| 54 | Best Of Both WorldsLulu | 54 | Chart history → |
| 55 | Born FreeThe Hesitations | 56 | Chart history → |
| 56 | There IsThe Dells | 66 | Chart history → |
| 57 | I Can't Stand Myself (When You Touch Me)James Brown And The Famous Flames | 36 | Chart history → |
| 58 | Simon Says1910 Fruitgum Co. | 77 | Chart history → |
| 59 | Oh, How It HurtsBarbara Mason | 59 | Chart history → |
| 60 | I Thank YouSam & Dave | 72 | Chart history → |
| 61 | There Was A TimeJames Brown And The Famous Flames | 65 | Chart history → |
| 62 | Everything That Touches YouThe Association | — | Chart history → |
| 63 | Mission-ImpossibleLalo Schifrin | 78 | Chart history → |
| 64 | Sunshine Of Your LoveCream | 69 | Chart history → |
| 65 | Honey ChileMartha Reeves & The Vandellas | 38 | Chart history → |
| 66 | Get Out NowTommy James And The Shondells | 81 | Chart history → |
| 67 | Guitar ManElvis Presley | 83 | Chart history → |
| 68 | Hey Little OneGlen Campbell | 70 | Chart history → |
| 69 | Who Will Answer?Ed Ames | 46 | Chart history → |
| 70 | I'm In LoveWilson Pickett | 58 | Chart history → |
| 71 | Walk Away ReneeFour Tops | — | Chart history → |
| 72 | Everybody KnowsThe Dave Clark Five | 43 | Chart history → |
| 73 | Do Unto MeJames & Bobby Purify | 73 | Chart history → |
| 74 | A Working Man's PrayerArthur Prysock | 74 | Chart history → |
| 75 | Come See About MeJr. Walker & The All Stars | 27 | Chart history → |
| 76 | WindyWes Montgomery | 53 | Chart history → |
| 77 | Pick Up The PiecesCarla Thomas | 68 | Chart history → |
| 78 | United (Part 1)The Music Makers | 79 | Chart history → |
| 79 | LostJerry Butler | 62 | Chart history → |
| 80 | A Man Needs A WomanJames Carr | 80 | Chart history → |
| 81 | A Million To OneFive Stairsteps & Cubie | 84 | Chart history → |
| 82 | StopHoward Tate | 82 | Chart history → |
| 83 | Looking For A FoxClarence Carter | 88 | Chart history → |
| 84 | Cab DriverThe Mills Brothers | 92 | Chart history → |
| 85 | MalayishaMiriam Makeba | 85 | Chart history → |
| 86 | (1-2-3-4-5-6-7) Count The DaysInez & Charlie Foxx | 76 | Chart history → |
| 87 | Cold FeetAlbert King | — | Chart history → |
| 88 | Burning SpearThe Soulful Strings | — | Chart history → |
| 89 | Funky WayCalvin Arnold | 89 | Chart history → |
| 90 | Try ItOhio Express | — | Chart history → |
| 91 | Rosanna's Going WildJohnny Cash | 91 | Chart history → |
| 92 | La - La - Means I Love YouThe Delfonics | — | Chart history → |
| 93 | Give My Love A TryLinda Jones | 94 | Chart history → |
| 94 | To Each His OwnFrankie Laine | 95 | Chart history → |
| 95 | People WorldJim & Jean | — | Chart history → |
| 96 | 7:30 Guided TourThe Five Americans | 96 | Chart history → |
| 97 | Carpet ManThe 5th Dimension | — | Chart history → |
| 98 | It's Not EasyThe Will-O-Bees | — | Chart history → |
| 99 | No One KnowsEvery Mothers' Son | 99 | Chart history → |
| 100 | (You've Got) Personality And Chantilly LaceMitch Ryder | — | Chart history → |