| 1 | HoneyBobby Goldsboro | 1 | Chart history → |
| 2 | Tighten UpArchie Bell & The Drells | 5 | Chart history → |
| 3 | Young GirlThe Union Gap Featuring Gary Puckett | 3 | Chart history → |
| 4 | The Good, The Bad And The UglyHugo Montenegro, His Orchestra And Chorus | 8 | Chart history → |
| 5 | Cry Like A BabyThe Box Tops | 2 | Chart history → |
| 6 | A Beautiful MorningThe Rascals | 9 | Chart history → |
| 7 | Cowboys To GirlsThe Intruders | 7 | Chart history → |
| 8 | The UnicornThe Irish Rovers | 10 | Chart history → |
| 9 | Mrs. RobinsonSimon & Garfunkel | 32 | Chart history → |
| 10 | Lady MadonnaThe Beatles | 4 | Chart history → |
| 11 | Love Is All AroundThe Troggs | 17 | Chart history → |
| 12 | I Got The Feelin'James Brown And The Famous Flames | 6 | Chart history → |
| 13 | Take Time To Know HerPercy Sledge | 13 | Chart history → |
| 14 | Funky StreetArthur Conley | 23 | Chart history → |
| 15 | Summertime BluesBlue Cheer | 14 | Chart history → |
| 16 | Ain't No WayAretha Franklin | 16 | Chart history → |
| 17 | The Ballad Of Bonnie And ClydeGeorgie Fame | 15 | Chart history → |
| 18 | Sweet InspirationThe Sweet Inspirations | 18 | Chart history → |
| 19 | Do You Know The Way To San JoséDionne Warwick | 21 | Chart history → |
| 20 | Shoo-Be-Doo-Be-Doo-Da-DayStevie Wonder | 20 | Chart history → |
| 21 | Dance To The MusicSly & The Family Stone | 12 | Chart history → |
| 22 | Mony MonyTommy James And The Shondells | 34 | Chart history → |
| 23 | Soul SerenadeWillie Mitchell | 30 | Chart history → |
| 24 | Ain't Nothing Like The Real ThingMarvin Gaye & Tammi Terrell | 25 | Chart history → |
| 25 | (Sweet Sweet Baby) Since You've Been GoneAretha Franklin | 22 | Chart history → |
| 26 | PlayboyGene And Debbe | 24 | Chart history → |
| 27 | DelilahTom Jones | 27 | Chart history → |
| 28 | U.S. MaleElvis Presley With The Jordanaires | 31 | Chart history → |
| 29 | I Will Always Think About YouThe New Colony Six | 44 | Chart history → |
| 30 | She's Lookin' GoodWilson Pickett | 41 | Chart history → |
| 31 | Mighty Quinn (Quinn The Eskimo)Manfred Mann | 29 | Chart history → |
| 32 | La - La - Means I Love YouThe Delfonics | 26 | Chart history → |
| 33 | If You Can WantSmokey Robinson & The Miracles | 11 | Chart history → |
| 34 | Take Good Care Of My BabyBobby Vinton | 33 | Chart history → |
| 35 | (Sittin' On) The Dock Of The BayOtis Redding | 19 | Chart history → |
| 36 | If I Were A CarpenterFour Tops | 69 | Chart history → |
| 37 | The Happy Song (Dum-Dum)Otis Redding | 47 | Chart history → |
| 38 | Scarborough Fair (/Canticle)Simon & Garfunkel | 36 | Chart history → |
| 39 | The Unknown SoldierThe Doors | 39 | Chart history → |
| 40 | Call Me LightningThe Who | 40 | Chart history → |
| 41 | Jennifer EcclesThe Hollies | 43 | Chart history → |
| 42 | The Son Of Hickory Holler's TrampO.C. Smith | 42 | Chart history → |
| 43 | Master JackFour Jacks And A Jill | 63 | Chart history → |
| 44 | Forever Came TodayDiana Ross & The Supremes | 28 | Chart history → |
| 45 | Like To Get To Know YouSpanky And Our Gang | 46 | Chart history → |
| 46 | Does Your Mama Know About MeBobby Taylor & The Vancouvers | 48 | Chart history → |
| 47 | ValleriThe Monkees | 45 | Chart history → |
| 48 | My Girl/Hey GirlBobby Vee | 49 | Chart history → |
| 49 | Look To Your SoulJohnny Rivers | 50 | Chart history → |
| 50 | Ame Caline (Soul Coaxing)Raymond Lefevre and His Orchestra | 37 | Chart history → |
| 51 | Loving You Has Made Me BananasGuy Marks | 51 | Chart history → |
| 52 | Paying The Cost To Be The BossB.B. King | 54 | Chart history → |
| 53 | Wear It On Our FaceThe Dells | 62 | Chart history → |
| 54 | I Wanna LiveGlen Campbell | 61 | Chart history → |
| 55 | FriendsThe Beach Boys | 66 | Chart history → |
| 56 | I Could Never Love Another (After Loving You)The Temptations | 87 | Chart history → |
| 57 | JumboBee Gees | 57 | Chart history → |
| 58 | Foggy Mountain BreakdownFlatt & Scruggs | 55 | Chart history → |
| 59 | We're Rolling On (Part I)The Impressions | 59 | Chart history → |
| 60 | I Can't Believe I'm Losing YouFrank Sinatra | 65 | Chart history → |
| 61 | I Love YouPeople | 85 | Chart history → |
| 62 | Yummy Yummy YummyOhio Express | 88 | Chart history → |
| 63 | Goodbye Baby (I Don't Want To See You Cry)Tommy Boyce & Bobby Hart | 53 | Chart history → |
| 64 | If You Don't Want My LoveRobert John | 76 | Chart history → |
| 65 | Baby Make Your Own Sweet MusicJay And The Techniques | 73 | Chart history → |
| 66 | I Promise To Wait My LoveMartha Reeves & The Vandellas | 78 | Chart history → |
| 67 | Funky Walk Part I (East)Dyke And The Blazers | 70 | Chart history → |
| 68 | Impossible Mission (Mission Impossible)Soul Survivors | 71 | Chart history → |
| 69 | I'm SorryThe Delfonics | 77 | Chart history → |
| 70 | Sherry Don't GoThe Lettermen | 64 | Chart history → |
| 71 | UnwindRay Stevens | 75 | Chart history → |
| 72 | L. David SloaneMichele Lee | 72 | Chart history → |
| 73 | (You Keep Me) Hangin' OnJoe Simon | 82 | Chart history → |
| 74 | I Got A Sure ThingOllie & The Nightingales | 74 | Chart history → |
| 75 | May I Take A Giant Step (Into Your Heart)1910 Fruitgum Co. | 83 | Chart history → |
| 76 | CabaretHerb Alpert & The Tijuana Brass | 81 | Chart history → |
| 77 | The Look Of LoveSergio Mendes & Brasil '66 | — | Chart history → |
| 78 | I Can RememberJames & Bobby Purify | 94 | Chart history → |
| 79 | MacArthur ParkRichard Harris | — | Chart history → |
| 80 | How'd We Ever Get This WayAndy Kim | 100 | Chart history → |
| 81 | Love In Every RoomPaul Mauriat And His Orchestra | — | Chart history → |
| 82 | Here's To YouHamilton Camp | 99 | Chart history → |
| 83 | Angel Of The MorningMerrilee Rush & The Turnabouts | 97 | Chart history → |
| 84 | Gentle On My MindPatti Page | 84 | Chart history → |
| 85 | Never Give You UpJerry Butler | 91 | Chart history → |
| 86 | Chain GangJackie Wilson & Count Basie | 86 | Chart history → |
| 87 | A Man Without Love (Quando M'innamoro)Engelbert Humperdinck | — | Chart history → |
| 88 | I Wish I Knew (How It Would Feel To Be Free)Solomon Burke | 95 | Chart history → |
| 89 | A Tribute To A KingWilliam Bell | 89 | Chart history → |
| 90 | Soul TrainClassics IV | 90 | Chart history → |
| 91 | I Have A DreamRev. Martin Luther King, Jr. | 92 | Chart history → |
| 92 | He Don't Really Love YouThe Delfonics | 93 | Chart history → |
| 93 | You Ain't Going NowhereThe Byrds | — | Chart history → |
| 94 | Lili MarleneAl Martino | 96 | Chart history → |
| 95 | Sleepy JoeHerman's Hermits | — | Chart history → |
| 96 | Face It Girl, It's OverNancy Wilson | — | Chart history → |
| 97 | ApologizeEd Ames | — | Chart history → |
| 98 | Brooklyn RoadsNeil Diamond | — | Chart history → |
| 99 | Anyone For TennisCream | — | Chart history → |
| 100 | She's A HeartbreakerGene Pitney | — | Chart history → |