| 1 | Tighten UpArchie Bell & The Drells | 1 | Chart history → |
| 2 | Mrs. RobinsonSimon & Garfunkel | 2 | Chart history → |
| 3 | A Beautiful MorningThe Rascals | 5 | Chart history → |
| 4 | The Good, The Bad And The UglyHugo Montenegro, His Orchestra And Chorus | 4 | Chart history → |
| 5 | HoneyBobby Goldsboro | 3 | Chart history → |
| 6 | Cowboys To GirlsThe Intruders | 6 | Chart history → |
| 7 | The UnicornThe Irish Rovers | 8 | Chart history → |
| 8 | Ain't Nothing Like The Real ThingMarvin Gaye & Tammi Terrell | 14 | Chart history → |
| 9 | Shoo-Be-Doo-Be-Doo-Da-DayStevie Wonder | 11 | Chart history → |
| 10 | Do You Know The Way To San JoséDionne Warwick | 10 | Chart history → |
| 11 | Take Time To Know HerPercy Sledge | 13 | Chart history → |
| 12 | Mony MonyTommy James And The Shondells | 19 | Chart history → |
| 13 | Young GirlThe Union Gap Featuring Gary Puckett | 9 | Chart history → |
| 14 | Love Is All AroundThe Troggs | 7 | Chart history → |
| 15 | She's Lookin' GoodWilson Pickett | 22 | Chart history → |
| 16 | ThinkAretha Franklin | 67 | Chart history → |
| 17 | I Got The Feelin'James Brown And The Famous Flames | 17 | Chart history → |
| 18 | Funky StreetArthur Conley | 18 | Chart history → |
| 19 | Cry Like A BabyThe Box Tops | 12 | Chart history → |
| 20 | Like To Get To Know YouSpanky And Our Gang | 20 | Chart history → |
| 21 | DelilahTom Jones | 26 | Chart history → |
| 22 | I Could Never Love Another (After Loving You)The Temptations | 25 | Chart history → |
| 23 | Soul SerenadeWillie Mitchell | 23 | Chart history → |
| 24 | Yummy Yummy YummyOhio Express | 32 | Chart history → |
| 25 | The Happy Song (Dum-Dum)Otis Redding | 27 | Chart history → |
| 26 | If I Were A CarpenterFour Tops | 29 | Chart history → |
| 27 | This Guy's In Love With YouHerb Alpert | 72 | Chart history → |
| 28 | I Will Always Think About YouThe New Colony Six | 28 | Chart history → |
| 29 | Does Your Mama Know About MeBobby Taylor & The Vancouvers | 30 | Chart history → |
| 30 | Master JackFour Jacks And A Jill | 31 | Chart history → |
| 31 | Lady MadonnaThe Beatles | 15 | Chart history → |
| 32 | Sweet InspirationThe Sweet Inspirations | 24 | Chart history → |
| 33 | Summertime BluesBlue Cheer | 16 | Chart history → |
| 34 | MacArthur ParkRichard Harris | 48 | Chart history → |
| 35 | My Girl/Hey GirlBobby Vee | 36 | Chart history → |
| 36 | I Wanna LiveGlen Campbell | 44 | Chart history → |
| 37 | Ain't No WayAretha Franklin | 21 | Chart history → |
| 38 | PlayboyGene And Debbe | 38 | Chart history → |
| 39 | Paying The Cost To Be The BossB.B. King | 52 | Chart history → |
| 40 | I Love YouPeople | 50 | Chart history → |
| 41 | (You Keep Me) Hangin' OnJoe Simon | 61 | Chart history → |
| 42 | The Look Of LoveSergio Mendes & Brasil '66 | 60 | Chart history → |
| 43 | I'm SorryThe Delfonics | 46 | Chart history → |
| 44 | Wear It On Our FaceThe Dells | 45 | Chart history → |
| 45 | The Son Of Hickory Holler's TrampO.C. Smith | 43 | Chart history → |
| 46 | Time For Livin'The Association | 73 | Chart history → |
| 47 | FriendsThe Beach Boys | 47 | Chart history → |
| 48 | Angel Of The MorningMerrilee Rush & The Turnabouts | 55 | Chart history → |
| 49 | How'd We Ever Get This WayAndy Kim | 54 | Chart history → |
| 50 | Never Give You UpJerry Butler | 62 | Chart history → |
| 51 | I Can RememberJames & Bobby Purify | 51 | Chart history → |
| 52 | A Man Without Love (Quando M'innamoro)Engelbert Humperdinck | 53 | Chart history → |
| 53 | If You Don't Want My LoveRobert John | 57 | Chart history → |
| 54 | Jennifer EcclesThe Hollies | 40 | Chart history → |
| 55 | UnwindRay Stevens | 56 | Chart history → |
| 56 | Jelly Jungle (Of Orange Marmalade)Lemon Pipers | 70 | Chart history → |
| 57 | Reach Out Of The DarknessFriend And Lover | 97 | Chart history → |
| 58 | She's A HeartbreakerGene Pitney | 65 | Chart history → |
| 59 | UnitedPeaches & Herb | 89 | Chart history → |
| 60 | Love In Every RoomPaul Mauriat And His Orchestra | 71 | Chart history → |
| 61 | I'll Never Do You WrongJoe Tex | 81 | Chart history → |
| 62 | I Promise To Wait My LoveMartha Reeves & The Vandellas | 66 | Chart history → |
| 63 | We're Rolling On (Part I)The Impressions | 63 | Chart history → |
| 64 | Baby Make Your Own Sweet MusicJay And The Techniques | 64 | Chart history → |
| 65 | Anyone For TennisCream | 79 | Chart history → |
| 66 | Brooklyn RoadsNeil Diamond | 75 | Chart history → |
| 67 | Sleepy JoeHerman's Hermits | 80 | Chart history → |
| 68 | May I Take A Giant Step (Into Your Heart)1910 Fruitgum Co. | 69 | Chart history → |
| 69 | Tip-Toe Thru' The Tulips With MeTiny Tim | 83 | Chart history → |
| 70 | Impossible Mission (Mission Impossible)Soul Survivors | 68 | Chart history → |
| 71 | The HorseCliff Nobles & Co. | — | Chart history → |
| 72 | CabaretHerb Alpert & The Tijuana Brass | 76 | Chart history → |
| 73 | I Got A Sure ThingOllie & The Nightingales | 74 | Chart history → |
| 74 | I Wish I Knew (How It Would Feel To Be Free)Solomon Burke | 77 | Chart history → |
| 75 | Licking Stick - Licking Stick (Part 1)James Brown And The Famous Flames | — | Chart history → |
| 76 | Here's To YouHamilton Camp | 82 | Chart history → |
| 77 | You Don't Know What You Mean To MeSam & Dave | — | Chart history → |
| 78 | You Ain't Going NowhereThe Byrds | 78 | Chart history → |
| 79 | I Got You BabeEtta James | 88 | Chart history → |
| 80 | My Shy VioletThe Mills Brothers | 84 | Chart history → |
| 81 | Face It Girl, It's OverNancy Wilson | 95 | Chart history → |
| 82 | ApologizeEd Ames | 94 | Chart history → |
| 83 | The DoctorMary Wells | 100 | Chart history → |
| 84 | Chain GangJackie Wilson & Count Basie | 85 | Chart history → |
| 85 | Gentle On My MindPatti Page | 87 | Chart history → |
| 86 | A Tribute To A KingWilliam Bell | 86 | Chart history → |
| 87 | Lili MarleneAl Martino | 93 | Chart history → |
| 88 | I Have A DreamRev. Martin Luther King, Jr. | 91 | Chart history → |
| 89 | America Is My Home - Pt. 1James Brown And The Famous Flames | — | Chart history → |
| 90 | Climb Every MountainThe Hesitations | — | Chart history → |
| 91 | It's OverEddy Arnold | 96 | Chart history → |
| 92 | He Don't Really Love YouThe Delfonics | 92 | Chart history → |
| 93 | Hold OnRadiants | — | Chart history → |
| 94 | Lonely Is The NameSammy Davis Jr. | — | Chart history → |
| 95 | I Can't Make It AloneBill Medley | 98 | Chart history → |
| 96 | Folsom Prison BluesJohnny Cash | — | Chart history → |
| 97 | Bring A Little Lovin'Los Bravos | — | Chart history → |
| 98 | Pictures Of Matchstick MenThe Status Quo | 99 | Chart history → |
| 99 | Don't Sign The Paper Baby (I Want You Back)Jimmy Delphs | — | Chart history → |
| 100 | Ready, Willing and AbleThe American Breed | — | Chart history → |