| 1 | I Heard It Through The GrapevineMarvin Gaye | 4 | Chart history → |
| 2 | Love ChildDiana Ross & The Supremes | 1 | Chart history → |
| 3 | For Once In My LifeStevie Wonder | 3 | Chart history → |
| 4 | Abraham, Martin And JohnDion | 7 | Chart history → |
| 5 | Who's Making LoveJohnnie Taylor | 5 | Chart history → |
| 6 | Hey JudeThe Beatles | 2 | Chart history → |
| 7 | Wichita LinemanGlen Campbell | 8 | Chart history → |
| 8 | StormyClassics IV Featuring Dennis Yost | 9 | Chart history → |
| 9 | I Love How You Love MeBobby Vinton | 11 | Chart history → |
| 10 | Magic Carpet RideSteppenwolf | 6 | Chart history → |
| 11 | Both Sides NowJudy Collins | 13 | Chart history → |
| 12 | Those Were The DaysMary Hopkin | 10 | Chart history → |
| 13 | Cloud NineThe Temptations | 15 | Chart history → |
| 14 | See SawAretha Franklin | 17 | Chart history → |
| 15 | Chewy ChewyOhio Express | 20 | Chart history → |
| 16 | Scarborough FairSergio Mendes & Brasil '66 | 26 | Chart history → |
| 17 | CinnamonDerek | 24 | Chart history → |
| 18 | Bring It On Home To MeEddie Floyd | 18 | Chart history → |
| 19 | Hold Me TightJohnny Nash | 12 | Chart history → |
| 20 | I'm Gonna Make You Love MeDiana Ross And The Supremes & The Temptations | 57 | Chart history → |
| 21 | Little ArrowsLeapy Lee | 16 | Chart history → |
| 22 | Promises, PromisesDionne Warwick | 19 | Chart history → |
| 23 | Hooked On A FeelingB.J. Thomas | 41 | Chart history → |
| 24 | Soulful StrutYoung-Holt Unlimited | 31 | Chart history → |
| 25 | Bang-Shang-A-LangThe Archies | 22 | Chart history → |
| 26 | White RoomCream | 14 | Chart history → |
| 27 | Pickin' Wild Mountain BerriesPeggy Scott & Jo Jo Benson | 27 | Chart history → |
| 28 | Too Weak To FightClarence Carter | 28 | Chart history → |
| 29 | TillThe Vogues | 35 | Chart history → |
| 30 | Shame, ShameMagic Lanterns | 30 | Chart history → |
| 31 | Goodbye My LoveJames Brown | 34 | Chart history → |
| 32 | Lo Mucho Que Te Quiero (The More I Love You)Rene & Rene | 44 | Chart history → |
| 33 | Papa's Got A Brand New BagOtis Redding | 50 | Chart history → |
| 34 | Quick Joey Small (Run Joey Run)Kasenetz-Katz Singing Orchestral Circus | 25 | Chart history → |
| 35 | CyclesFrank Sinatra | 29 | Chart history → |
| 36 | Son-Of-A Preacher ManDusty Springfield | 49 | Chart history → |
| 37 | Goody Goody Gumdrops1910 Fruitgum Co. | 40 | Chart history → |
| 38 | Kentucky WomanDeep Purple | 38 | Chart history → |
| 39 | A Ray Of HopeThe Rascals | 58 | Chart history → |
| 40 | If I Can DreamElvis Presley | 63 | Chart history → |
| 41 | Hang 'Em HighBooker T. & The MG's | 42 | Chart history → |
| 42 | A Man And A HalfWilson Pickett | 68 | Chart history → |
| 43 | Not Enough IndiansDean Martin | 43 | Chart history → |
| 44 | I Can't Turn You LooseThe Chambers Brothers | 45 | Chart history → |
| 45 | Battle Hymn Of The RepublicAndy Williams with the St. Charles Borromeo Choir | 33 | Chart history → |
| 46 | Put Your Head On My ShoulderThe Lettermen | 47 | Chart history → |
| 47 | Les Bicyclettes De BelsizeEngelbert Humperdinck | 39 | Chart history → |
| 48 | Ballad Of Two BrothersAutry Inman | 56 | Chart history → |
| 49 | The Straight LifeBobby Goldsboro | 36 | Chart history → |
| 50 | This Is My CountryThe Impressions | 69 | Chart history → |
| 51 | Stand By Your ManTammy Wynette | 67 | Chart history → |
| 52 | Going Up The CountryCanned Heat | 74 | Chart history → |
| 53 | PeopleThe Tymes | 54 | Chart history → |
| 54 | Slow DragThe Intruders | 55 | Chart history → |
| 55 | My SongAretha Franklin | 59 | Chart history → |
| 56 | ShakeShadows Of Knight | 46 | Chart history → |
| 57 | FireFive By Five | 52 | Chart history → |
| 58 | Bella LindaThe Grass Roots | 90 | Chart history → |
| 59 | I Put A Spell On YouCreedence Clearwater Revival | 72 | Chart history → |
| 60 | Talking About My BabyGloria Walker | 60 | Chart history → |
| 61 | Crosstown TrafficThe Jimi Hendrix Experience | 73 | Chart history → |
| 62 | American BoysPetula Clark | 75 | Chart history → |
| 63 | Come On, React!The Fireballs | 86 | Chart history → |
| 64 | Rockin' In The Same Old BoatBobby Bland | 65 | Chart history → |
| 65 | I Walk AloneMarty Robbins | 66 | Chart history → |
| 66 | Ready Or Not Here I Come (Can't Hide From Love)The Delfonics | 94 | Chart history → |
| 67 | MalindaBobby Taylor & The Vancouvers | 80 | Chart history → |
| 68 | With A Little Help From My FriendsJoe Cocker | 76 | Chart history → |
| 69 | Baby Let's WaitThe Royal Guardsmen | 83 | Chart history → |
| 70 | Just Ain't No LoveBarbara Acklin | 87 | Chart history → |
| 71 | Don't Cry My LoveThe Impressions | 71 | Chart history → |
| 72 | Everyday PeopleSly & The Family Stone | 78 | Chart history → |
| 73 | Keep On DancingAlvin Cash | 79 | Chart history → |
| 74 | Bluebirds Over The MountainThe Beach Boys | — | Chart history → |
| 75 | My Favorite ThingsHerb Alpert & The Tijuana Brass | — | Chart history → |
| 76 | Do You Wanna DanceThe Mamas & The Papas | 88 | Chart history → |
| 77 | Love MachineThe O'Kaysions | 77 | Chart history → |
| 78 | Are You HappyJerry Butler | 96 | Chart history → |
| 79 | Don't Make The Good Girls Go BadDella Humphrey | 92 | Chart history → |
| 80 | Isn't It Lonely TogetherO.C. Smith | — | Chart history → |
| 81 | Born To Be With YouSonny James | 81 | Chart history → |
| 82 | Chitty Chitty Bang BangPaul Mauriat | 82 | Chart history → |
| 83 | The Girl Most LikelyJeannie C. Riley | 85 | Chart history → |
| 84 | Good Time GirlNancy Sinatra | 91 | Chart history → |
| 85 | Crimson And CloverTommy James And The Shondells | — | Chart history → |
| 86 | The Beginning Of My EndThe Unifics | — | Chart history → |
| 87 | There's Gonna Be A ShowdownArchie Bell & The Drells | — | Chart history → |
| 88 | White HousesEric Burdon & The Animals | 93 | Chart history → |
| 89 | Reach OutMerrilee Rush | 89 | Chart history → |
| 90 | You Got SoulJohnny Nash | — | Chart history → |
| 91 | Looking BackJoe Simon | 98 | Chart history → |
| 92 | California Dreamin'Bobby Womack | 97 | Chart history → |
| 93 | Don't Be Afraid (Do As I Say)Frankie Karl & The Dreams | — | Chart history → |
| 94 | I've Gotta Be MeSammy Davis Jr. | — | Chart history → |
| 95 | Yesterday's RainSpanky And Our Gang | 95 | Chart history → |
| 96 | Release MeJohnny Adams | — | Chart history → |
| 97 | The WormJimmy McGriff | — | Chart history → |
| 98 | Don't Pat Me On The Back And Call Me BrotherJohn W. Anderson presents KaSandra | — | Chart history → |
| 99 | They Don't Make Love Like They Used ToEddy Arnold | 99 | Chart history → |
| 100 | VanceRoger Miller | 100 | Chart history → |