| 1 | Love Is Blue (L'amour Est Bleu)Paul Mauriat And His Orchestra | 1 | Chart history → |
| 2 | (Theme From) Valley Of The DollsDionne Warwick | 2 | Chart history → |
| 3 | (Sittin' On) The Dock Of The BayOtis Redding | 5 | Chart history → |
| 4 | I Wish It Would RainThe Temptations | 4 | Chart history → |
| 5 | Simon Says1910 Fruitgum Co. | 6 | Chart history → |
| 6 | SpookyClassics IV | 3 | Chart history → |
| 7 | Just Dropped In (To See What Condition My Condition Was In)The First Edition | 21 | Chart history → |
| 8 | I Wonder What She's Doing ToniteTommy Boyce & Bobby Hart | 8 | Chart history → |
| 9 | Bottle Of WineThe Fireballs | 12 | Chart history → |
| 10 | Everything That Touches YouThe Association | 15 | Chart history → |
| 11 | Baby, Now That I've Found YouThe Foundations | 11 | Chart history → |
| 12 | Nobody But MeThe Human Beinz | 10 | Chart history → |
| 13 | Goin' Out Of My Head/Can't Take My Eyes Off YouThe Lettermen | 9 | Chart history → |
| 14 | Green TambourineThe Lemon Pipers | 7 | Chart history → |
| 15 | WordsBee Gees | 16 | Chart history → |
| 16 | We're A WinnerThe Impressions | 14 | Chart history → |
| 17 | Walk Away ReneeFour Tops | 19 | Chart history → |
| 18 | Judy In Disguise (With Glasses)John Fred And The Playboys | 13 | Chart history → |
| 19 | La - La - Means I Love YouThe Delfonics | 35 | Chart history → |
| 20 | There IsThe Dells | 20 | Chart history → |
| 21 | I Thank YouSam & Dave | 24 | Chart history → |
| 22 | Bend Me, Shape MeThe American Breed | 18 | Chart history → |
| 23 | I Can Take Or Leave Your LovingHerman's Hermits | 22 | Chart history → |
| 24 | Woman, WomanThe Union Gap Featuring Gary Puckett | 17 | Chart history → |
| 25 | Too Much TalkPaul Revere & The Raiders Featuring Mark Lindsay | 34 | Chart history → |
| 26 | The End Of Our RoadGladys Knight And The Pips | 30 | Chart history → |
| 27 | We Can FlyThe Cowsills | 23 | Chart history → |
| 28 | Itchycoo ParkSmall Faces | 27 | Chart history → |
| 29 | Skip A RopeHenson Cargill | 26 | Chart history → |
| 30 | The Ballad Of Bonnie And ClydeGeorgie Fame | 49 | Chart history → |
| 31 | (Sweet Sweet Baby) Since You've Been GoneAretha Franklin | — | Chart history → |
| 32 | Different DrumStone Poneys Featuring Linda Ronstadt | 29 | Chart history → |
| 33 | TomorrowStrawberry Alarm Clock | 32 | Chart history → |
| 34 | Dance To The MusicSly & The Family Stone | 41 | Chart history → |
| 35 | Kiss Me GoodbyePetula Clark | 52 | Chart history → |
| 36 | Sunshine Of Your LoveCream | 37 | Chart history → |
| 37 | Carpet ManThe 5th Dimension | 40 | Chart history → |
| 38 | Cab DriverThe Mills Brothers | 50 | Chart history → |
| 39 | There Was A TimeJames Brown And The Famous Flames | 36 | Chart history → |
| 40 | Men Are Gettin' ScarceJoe Tex | 44 | Chart history → |
| 41 | Mission-ImpossibleLalo Schifrin | 42 | Chart history → |
| 42 | Born FreeThe Hesitations | 38 | Chart history → |
| 43 | Guitar ManElvis Presley | 43 | Chart history → |
| 44 | Will You Love Me TomorrowThe 4 Seasons Featuring the "Sound of Frankie Valli" | 78 | Chart history → |
| 45 | PlayboyGene And Debbe | 60 | Chart history → |
| 46 | I'm Gonna Make You Love MeMadeline Bell | 51 | Chart history → |
| 47 | If You Can WantSmokey Robinson & The Miracles | 85 | Chart history → |
| 48 | Country Girl - City ManBilly Vera & Judy Clay | 55 | Chart history → |
| 49 | Get Out NowTommy James And The Shondells | 48 | Chart history → |
| 50 | Jealous LoveWilson Pickett | 59 | Chart history → |
| 51 | Suddenly You Love MeThe Tremeloes | 71 | Chart history → |
| 52 | For Your Precious LoveJackie Wilson & Count Basie | 64 | Chart history → |
| 53 | Maybe Just TodayBobby Vee And The Strangers | 53 | Chart history → |
| 54 | A Question Of TemperatureThe Balloon Farm | 66 | Chart history → |
| 55 | In The Midnight HourThe Mirettes | 61 | Chart history → |
| 56 | Look, Here Comes The SunThe Sunshine Company | 56 | Chart history → |
| 57 | Love Is BlueAl Martino | 57 | Chart history → |
| 58 | Got What You NeedThe Fantastic Johnny C | 58 | Chart history → |
| 59 | Hey Little OneGlen Campbell | 54 | Chart history → |
| 60 | Cry Like A BabyThe Box Tops | — | Chart history → |
| 61 | Scarborough Fair (/Canticle)Simon & Garfunkel | — | Chart history → |
| 62 | Looking For A FoxClarence Carter | 62 | Chart history → |
| 63 | A Man Needs A WomanJames Carr | 63 | Chart history → |
| 64 | Green LightThe American Breed | 90 | Chart history → |
| 65 | Little Green ApplesRoger Miller | — | Chart history → |
| 66 | The Good, The Bad And The UglyHugo Montenegro, His Orchestra And Chorus | 77 | Chart history → |
| 67 | Lovey DoveyOtis & Carla | 74 | Chart history → |
| 68 | Mighty Quinn (Quinn The Eskimo)Manfred Mann | — | Chart history → |
| 69 | Thank U Very MuchThe Scaffold | 70 | Chart history → |
| 70 | The Ten Commandments Of LovePeaches & Herb | 80 | Chart history → |
| 71 | A Million To OneFive Stairsteps & Cubie | 68 | Chart history → |
| 72 | I Say LoveThe Royal Guardsmen | 73 | Chart history → |
| 73 | Where Is My MindThe Vanilla Fudge | 83 | Chart history → |
| 74 | Here Comes The Rain, BabyEddy Arnold | 75 | Chart history → |
| 75 | Burning SpearThe Soulful Strings | 69 | Chart history → |
| 76 | Funky WayCalvin Arnold | 72 | Chart history → |
| 77 | That's A LieRay Charles | 86 | Chart history → |
| 78 | Night Fo' LastShorty Long | 79 | Chart history → |
| 79 | Hey Hey BunnyJohn Fred And The Playboys | 89 | Chart history → |
| 80 | The Son Of Hickory Holler's TrampO.C. Smith | 88 | Chart history → |
| 81 | If This World Were MineMarvin Gaye & Tammi Terrell | — | Chart history → |
| 82 | Ame Caline (Soul Coaxing)Raymond Lefevre and His Orchestra | 99 | Chart history → |
| 83 | SoulvilleAretha Franklin | 84 | Chart history → |
| 84 | SecurityEtta James | — | Chart history → |
| 85 | Love Is All AroundThe Troggs | 98 | Chart history → |
| 86 | L. David SloaneMichele Lee | — | Chart history → |
| 87 | Young GirlThe Union Gap Featuring Gary Puckett | — | Chart history → |
| 88 | Sweet InspirationThe Sweet Inspirations | — | Chart history → |
| 89 | Summertime BluesBlue Cheer | — | Chart history → |
| 90 | Sound AsleepThe Turtles | — | Chart history → |
| 91 | Funky North PhillyBill Cosby | — | Chart history → |
| 92 | Love ExplosionTroy Keyes | 93 | Chart history → |
| 93 | Gentle On My MindPatti Page | 95 | Chart history → |
| 94 | Springfield PlaneKenny O'Dell | 94 | Chart history → |
| 95 | Foggy Mountain BreakdownFlatt & Scruggs | — | Chart history → |
| 96 | Love Is Blue (L'Amour Est Bleu)Manny Kellem - His Orchestra And Voices | 100 | Chart history → |
| 97 | Love Is Blue (L'Amour Est Bleu)Claudine Longet | 97 | Chart history → |
| 98 | Dear DelilahGrapefruit | — | Chart history → |
| 99 | Sally Was A Good Old GirlTrini Lopez | — | Chart history → |
| 100 | You've Got To Be LovedThe Montanas | — | Chart history → |