| 1 | Love Is Blue (L'amour Est Bleu)Paul Mauriat And His Orchestra | 1 | Chart history → |
| 2 | (Theme From) Valley Of The DollsDionne Warwick | 2 | Chart history → |
| 3 | (Sittin' On) The Dock Of The BayOtis Redding | 3 | Chart history → |
| 4 | Simon Says1910 Fruitgum Co. | 5 | Chart history → |
| 5 | I Wish It Would RainThe Temptations | 4 | Chart history → |
| 6 | Just Dropped In (To See What Condition My Condition Was In)The First Edition | 7 | Chart history → |
| 7 | SpookyClassics IV | 6 | Chart history → |
| 8 | I Wonder What She's Doing ToniteTommy Boyce & Bobby Hart | 8 | Chart history → |
| 9 | La - La - Means I Love YouThe Delfonics | 19 | Chart history → |
| 10 | Everything That Touches YouThe Association | 10 | Chart history → |
| 11 | I Thank YouSam & Dave | 21 | Chart history → |
| 12 | Baby, Now That I've Found YouThe Foundations | 11 | Chart history → |
| 13 | Bottle Of WineThe Fireballs | 9 | Chart history → |
| 14 | Walk Away ReneeFour Tops | 17 | Chart history → |
| 15 | The End Of Our RoadGladys Knight And The Pips | 26 | Chart history → |
| 16 | We're A WinnerThe Impressions | 16 | Chart history → |
| 17 | (Sweet Sweet Baby) Since You've Been GoneAretha Franklin | 31 | Chart history → |
| 18 | WordsBee Gees | 15 | Chart history → |
| 19 | Dance To The MusicSly & The Family Stone | 34 | Chart history → |
| 20 | Too Much TalkPaul Revere & The Raiders Featuring Mark Lindsay | 25 | Chart history → |
| 21 | Goin' Out Of My Head/Can't Take My Eyes Off YouThe Lettermen | 13 | Chart history → |
| 22 | Nobody But MeThe Human Beinz | 12 | Chart history → |
| 23 | There IsThe Dells | 20 | Chart history → |
| 24 | ValleriThe Monkees | — | Chart history → |
| 25 | Green TambourineThe Lemon Pipers | 14 | Chart history → |
| 26 | The Ballad Of Bonnie And ClydeGeorgie Fame | 30 | Chart history → |
| 27 | Kiss Me GoodbyePetula Clark | 35 | Chart history → |
| 28 | Will You Love Me TomorrowThe 4 Seasons Featuring the "Sound of Frankie Valli" | 44 | Chart history → |
| 29 | Carpet ManThe 5th Dimension | 37 | Chart history → |
| 30 | Judy In Disguise (With Glasses)John Fred And The Playboys | 18 | Chart history → |
| 31 | If You Can WantSmokey Robinson & The Miracles | 47 | Chart history → |
| 32 | We Can FlyThe Cowsills | 27 | Chart history → |
| 33 | Men Are Gettin' ScarceJoe Tex | 40 | Chart history → |
| 34 | I'm Gonna Make You Love MeMadeline Bell | 46 | Chart history → |
| 35 | Mighty Quinn (Quinn The Eskimo)Manfred Mann | 68 | Chart history → |
| 36 | Woman, WomanThe Union Gap Featuring Gary Puckett | 24 | Chart history → |
| 37 | Cab DriverThe Mills Brothers | 38 | Chart history → |
| 38 | There Was A TimeJames Brown And The Famous Flames | 39 | Chart history → |
| 39 | I Can Take Or Leave Your LovingHerman's Hermits | 23 | Chart history → |
| 40 | PlayboyGene And Debbe | 45 | Chart history → |
| 41 | Mission-ImpossibleLalo Schifrin | 41 | Chart history → |
| 42 | Scarborough Fair (/Canticle)Simon & Garfunkel | 61 | Chart history → |
| 43 | Sunshine Of Your LoveCream | 36 | Chart history → |
| 44 | A Question Of TemperatureThe Balloon Farm | 54 | Chart history → |
| 45 | Country Girl - City ManBilly Vera & Judy Clay | 48 | Chart history → |
| 46 | Skip A RopeHenson Cargill | 29 | Chart history → |
| 47 | In The Midnight HourThe Mirettes | 55 | Chart history → |
| 48 | Maybe Just TodayBobby Vee And The Strangers | 53 | Chart history → |
| 49 | For Your Precious LoveJackie Wilson & Count Basie | 52 | Chart history → |
| 50 | Jealous LoveWilson Pickett | 50 | Chart history → |
| 51 | Suddenly You Love MeThe Tremeloes | 51 | Chart history → |
| 52 | Young GirlThe Union Gap Featuring Gary Puckett | 87 | Chart history → |
| 53 | Cry Like A BabyThe Box Tops | 60 | Chart history → |
| 54 | Born FreeThe Hesitations | 42 | Chart history → |
| 55 | Green LightThe American Breed | 64 | Chart history → |
| 56 | Got What You NeedThe Fantastic Johnny C | 58 | Chart history → |
| 57 | Love Is BlueAl Martino | 57 | Chart history → |
| 58 | The Ten Commandments Of LovePeaches & Herb | 70 | Chart history → |
| 59 | Little Green ApplesRoger Miller | 65 | Chart history → |
| 60 | Lovey DoveyOtis & Carla | 67 | Chart history → |
| 61 | Look, Here Comes The SunThe Sunshine Company | 56 | Chart history → |
| 62 | Looking For A FoxClarence Carter | 62 | Chart history → |
| 63 | A Man Needs A WomanJames Carr | 63 | Chart history → |
| 64 | The Good, The Bad And The UglyHugo Montenegro, His Orchestra And Chorus | 66 | Chart history → |
| 65 | Get Out NowTommy James And The Shondells | 49 | Chart history → |
| 66 | Summertime BluesBlue Cheer | 89 | Chart history → |
| 67 | Love Is All AroundThe Troggs | 85 | Chart history → |
| 68 | The Son Of Hickory Holler's TrampO.C. Smith | 80 | Chart history → |
| 69 | Thank U Very MuchThe Scaffold | 69 | Chart history → |
| 70 | SecurityEtta James | 84 | Chart history → |
| 71 | That's A LieRay Charles | 77 | Chart history → |
| 72 | I Say LoveThe Royal Guardsmen | 72 | Chart history → |
| 73 | Tapioca TundraThe Monkees | — | Chart history → |
| 74 | Soul SerenadeWillie Mitchell | — | Chart history → |
| 75 | Night Fo' LastShorty Long | 78 | Chart history → |
| 76 | Hey Hey BunnyJohn Fred And The Playboys | 79 | Chart history → |
| 77 | Ame Caline (Soul Coaxing)Raymond Lefevre and His Orchestra | 82 | Chart history → |
| 78 | Sweet InspirationThe Sweet Inspirations | 88 | Chart history → |
| 79 | You've Got To Be LovedThe Montanas | 100 | Chart history → |
| 80 | If This World Were MineMarvin Gaye & Tammi Terrell | 81 | Chart history → |
| 81 | Sound AsleepThe Turtles | 90 | Chart history → |
| 82 | Where Is My MindThe Vanilla Fudge | 73 | Chart history → |
| 83 | SoulvilleAretha Franklin | 83 | Chart history → |
| 84 | Rice Is NiceThe Lemon Pipers | — | Chart history → |
| 85 | I'll Say Forever My LoveJimmy Ruffin | — | Chart history → |
| 86 | L. David SloaneMichele Lee | 86 | Chart history → |
| 87 | Love Is Blue (L'Amour Est Bleu)Claudine Longet | 97 | Chart history → |
| 88 | Jennifer JuniperDonovan | — | Chart history → |
| 89 | (Sittin' On) The Dock Of The BayKing Curtis & The Kingpins | — | Chart history → |
| 90 | Back On My Feet AgainThe Foundations | — | Chart history → |
| 91 | Funky North PhillyBill Cosby | 91 | Chart history → |
| 92 | Turn On Your Love LightThe Human Beinz | — | Chart history → |
| 93 | Gentle On My MindPatti Page | 93 | Chart history → |
| 94 | (You Can't Let The Boy Overpower) The Man In YouChuck Jackson | — | Chart history → |
| 95 | Foggy Mountain BreakdownFlatt & Scruggs | 95 | Chart history → |
| 96 | Driftin' BluesBobby Bland | — | Chart history → |
| 97 | (1-2-3-4-5-6-7) Count The DaysInez & Charlie Foxx | — | Chart history → |
| 98 | Have A Little FaithDavid Houston | — | Chart history → |
| 99 | Sally Was A Good Old GirlTrini Lopez | 99 | Chart history → |
| 100 | Lovey Dovey Kinda Lovin'Brenton Wood | — | Chart history → |