| 1 | (Sittin' On) The Dock Of The BayOtis Redding | 3 | Chart history → |
| 2 | (Theme From) Valley Of The DollsDionne Warwick | 2 | Chart history → |
| 3 | Love Is Blue (L'amour Est Bleu)Paul Mauriat And His Orchestra | 1 | Chart history → |
| 4 | Simon Says1910 Fruitgum Co. | 4 | Chart history → |
| 5 | Just Dropped In (To See What Condition My Condition Was In)The First Edition | 6 | Chart history → |
| 6 | I Wish It Would RainThe Temptations | 5 | Chart history → |
| 7 | La - La - Means I Love YouThe Delfonics | 9 | Chart history → |
| 8 | ValleriThe Monkees | 24 | Chart history → |
| 9 | (Sweet Sweet Baby) Since You've Been GoneAretha Franklin | 17 | Chart history → |
| 10 | I Thank YouSam & Dave | 11 | Chart history → |
| 11 | SpookyClassics IV | 7 | Chart history → |
| 12 | Everything That Touches YouThe Association | 10 | Chart history → |
| 13 | Bottle Of WineThe Fireballs | 13 | Chart history → |
| 14 | Walk Away ReneeFour Tops | 14 | Chart history → |
| 15 | The End Of Our RoadGladys Knight And The Pips | 15 | Chart history → |
| 16 | Dance To The MusicSly & The Family Stone | 19 | Chart history → |
| 17 | The Ballad Of Bonnie And ClydeGeorgie Fame | 26 | Chart history → |
| 18 | WordsBee Gees | 18 | Chart history → |
| 19 | Too Much TalkPaul Revere & The Raiders Featuring Mark Lindsay | 20 | Chart history → |
| 20 | I Wonder What She's Doing ToniteTommy Boyce & Bobby Hart | 8 | Chart history → |
| 21 | We're A WinnerThe Impressions | 16 | Chart history → |
| 22 | Kiss Me GoodbyePetula Clark | 27 | Chart history → |
| 23 | There IsThe Dells | 23 | Chart history → |
| 24 | Young GirlThe Union Gap Featuring Gary Puckett | 52 | Chart history → |
| 25 | Mighty Quinn (Quinn The Eskimo)Manfred Mann | 35 | Chart history → |
| 26 | Baby, Now That I've Found YouThe Foundations | 12 | Chart history → |
| 27 | Will You Love Me TomorrowThe 4 Seasons Featuring the "Sound of Frankie Valli" | 28 | Chart history → |
| 28 | Cry Like A BabyThe Box Tops | 53 | Chart history → |
| 29 | Scarborough Fair (/Canticle)Simon & Garfunkel | 42 | Chart history → |
| 30 | If You Can WantSmokey Robinson & The Miracles | 31 | Chart history → |
| 31 | Nobody But MeThe Human Beinz | 22 | Chart history → |
| 32 | Goin' Out Of My Head/Can't Take My Eyes Off YouThe Lettermen | 21 | Chart history → |
| 33 | Men Are Gettin' ScarceJoe Tex | 33 | Chart history → |
| 34 | I'm Gonna Make You Love MeMadeline Bell | 34 | Chart history → |
| 35 | Cab DriverThe Mills Brothers | 37 | Chart history → |
| 36 | Carpet ManThe 5th Dimension | 29 | Chart history → |
| 37 | PlayboyGene And Debbe | 40 | Chart history → |
| 38 | A Question Of TemperatureThe Balloon Farm | 44 | Chart history → |
| 39 | Green LightThe American Breed | 55 | Chart history → |
| 40 | Little Green ApplesRoger Miller | 59 | Chart history → |
| 41 | Sunshine Of Your LoveCream | 43 | Chart history → |
| 42 | Love Is All AroundThe Troggs | 67 | Chart history → |
| 43 | Country Girl - City ManBilly Vera & Judy Clay | 45 | Chart history → |
| 44 | I Can Take Or Leave Your LovingHerman's Hermits | 39 | Chart history → |
| 45 | Suddenly You Love MeThe Tremeloes | 51 | Chart history → |
| 46 | Maybe Just TodayBobby Vee And The Strangers | 48 | Chart history → |
| 47 | In The Midnight HourThe Mirettes | 47 | Chart history → |
| 48 | Mission-ImpossibleLalo Schifrin | 41 | Chart history → |
| 49 | Tapioca TundraThe Monkees | 73 | Chart history → |
| 50 | Ame Caline (Soul Coaxing)Raymond Lefevre and His Orchestra | 77 | Chart history → |
| 51 | Summertime BluesBlue Cheer | 66 | Chart history → |
| 52 | The Son Of Hickory Holler's TrampO.C. Smith | 68 | Chart history → |
| 53 | The Good, The Bad And The UglyHugo Montenegro, His Orchestra And Chorus | 64 | Chart history → |
| 54 | For Your Precious LoveJackie Wilson & Count Basie | 49 | Chart history → |
| 55 | The Ten Commandments Of LovePeaches & Herb | 58 | Chart history → |
| 56 | Jealous LoveWilson Pickett | 50 | Chart history → |
| 57 | Love Is BlueAl Martino | 57 | Chart history → |
| 58 | Hey Hey BunnyJohn Fred And The Playboys | 76 | Chart history → |
| 59 | Sound AsleepThe Turtles | 81 | Chart history → |
| 60 | You've Got To Be LovedThe Montanas | 79 | Chart history → |
| 61 | Jennifer JuniperDonovan | 88 | Chart history → |
| 62 | Got What You NeedThe Fantastic Johnny C | 56 | Chart history → |
| 63 | I Got The Feelin'James Brown And The Famous Flames | — | Chart history → |
| 64 | Lovey DoveyOtis & Carla | 60 | Chart history → |
| 65 | Rice Is NiceThe Lemon Pipers | 84 | Chart history → |
| 66 | That's A LieRay Charles | 71 | Chart history → |
| 67 | SecurityEtta James | 70 | Chart history → |
| 68 | Soul SerenadeWillie Mitchell | 74 | Chart history → |
| 69 | Back On My Feet AgainThe Foundations | 90 | Chart history → |
| 70 | Forever Came TodayDiana Ross & The Supremes | — | Chart history → |
| 71 | If This World Were MineMarvin Gaye & Tammi Terrell | 80 | Chart history → |
| 72 | Sweet InspirationThe Sweet Inspirations | 78 | Chart history → |
| 73 | L. David SloaneMichele Lee | 86 | Chart history → |
| 74 | Take Time To Know HerPercy Sledge | — | Chart history → |
| 75 | Sit With The GuruStrawberry Alarm Clock | — | Chart history → |
| 76 | Jennifer EcclesThe Hollies | — | Chart history → |
| 77 | Funky StreetArthur Conley | — | Chart history → |
| 78 | Tin SoldierSmall Faces | — | Chart history → |
| 79 | Love Is Blue (L'Amour Est Bleu)Claudine Longet | 87 | Chart history → |
| 80 | Foggy Mountain BreakdownFlatt & Scruggs | 95 | Chart history → |
| 81 | I'll Say Forever My LoveJimmy Ruffin | 85 | Chart history → |
| 82 | Where Is My MindThe Vanilla Fudge | 82 | Chart history → |
| 83 | Stay AwayElvis Presley With The Jordanaires | — | Chart history → |
| 84 | In Need Of A FriendThe Cowsills | — | Chart history → |
| 85 | Turn On Your Love LightThe Human Beinz | 92 | Chart history → |
| 86 | (Sittin' On) The Dock Of The BayKing Curtis & The Kingpins | 89 | Chart history → |
| 87 | Baby You're So Right For MeBrenda & The Tabulations | — | Chart history → |
| 88 | 1941Tom Northcott | — | Chart history → |
| 89 | At The Top Of The StairsThe Formations | — | Chart history → |
| 90 | The Impossible DreamThe Hesitations | — | Chart history → |
| 91 | Funky North PhillyBill Cosby | 91 | Chart history → |
| 92 | The Father Of GirlsPerry Como | — | Chart history → |
| 93 | Gentle On My MindPatti Page | 93 | Chart history → |
| 94 | Up From The SkiesThe Jimi Hendrix Experience | — | Chart history → |
| 95 | Dr. Jon (The Medicine Man)Jon & Robin And The In Crowd | — | Chart history → |
| 96 | Driftin' BluesBobby Bland | 96 | Chart history → |
| 97 | DelilahTom Jones | — | Chart history → |
| 98 | Have A Little FaithDavid Houston | 98 | Chart history → |
| 99 | Lovey Dovey Kinda Lovin'Brenton Wood | 100 | Chart history → |
| 100 | In Some TimeRonnie Dove | — | Chart history → |