| 1 | Mrs. RobinsonSimon & Garfunkel | 1 | Chart history → |
| 2 | Tighten UpArchie Bell & The Drells | 4 | Chart history → |
| 3 | This Guy's In Love With YouHerb Alpert | 11 | Chart history → |
| 4 | The Good, The Bad And The UglyHugo Montenegro, His Orchestra And Chorus | 2 | Chart history → |
| 5 | Mony MonyTommy James And The Shondells | 7 | Chart history → |
| 6 | Yummy Yummy YummyOhio Express | 6 | Chart history → |
| 7 | MacArthur ParkRichard Harris | 12 | Chart history → |
| 8 | A Beautiful MorningThe Rascals | 3 | Chart history → |
| 9 | ThinkAretha Franklin | 13 | Chart history → |
| 10 | HoneyBobby Goldsboro | 5 | Chart history → |
| 11 | Ain't Nothing Like The Real ThingMarvin Gaye & Tammi Terrell | 8 | Chart history → |
| 12 | Cowboys To GirlsThe Intruders | 9 | Chart history → |
| 13 | The Look Of LoveSergio Mendes & Brasil '66 | 34 | Chart history → |
| 14 | Angel Of The MorningMerrilee Rush & The Turnabouts | 30 | Chart history → |
| 15 | DelilahTom Jones | 21 | Chart history → |
| 16 | Shoo-Be-Doo-Be-Doo-Da-DayStevie Wonder | 16 | Chart history → |
| 17 | Like To Get To Know YouSpanky And Our Gang | 19 | Chart history → |
| 18 | Master JackFour Jacks And A Jill | 23 | Chart history → |
| 19 | I Could Never Love Another (After Loving You)The Temptations | 20 | Chart history → |
| 20 | If I Were A CarpenterFour Tops | 25 | Chart history → |
| 21 | Do You Know The Way To San JoséDionne Warwick | 10 | Chart history → |
| 22 | I Love YouPeople | 31 | Chart history → |
| 23 | Reach Out Of The DarknessFriend And Lover | 38 | Chart history → |
| 24 | Take Time To Know HerPercy Sledge | 24 | Chart history → |
| 25 | Licking Stick - Licking Stick (Part 1)James Brown And The Famous Flames | 32 | Chart history → |
| 26 | I Will Always Think About YouThe New Colony Six | 22 | Chart history → |
| 27 | A Man Without Love (Quando M'innamoro)Engelbert Humperdinck | 39 | Chart history → |
| 28 | The Happy Song (Dum-Dum)Otis Redding | 28 | Chart history → |
| 29 | How'd We Ever Get This WayAndy Kim | 29 | Chart history → |
| 30 | She's Lookin' GoodWilson Pickett | 15 | Chart history → |
| 31 | Love Is All AroundThe Troggs | 14 | Chart history → |
| 32 | Soul SerenadeWillie Mitchell | 26 | Chart history → |
| 33 | Tip-Toe Thru' The Tulips With MeTiny Tim | 46 | Chart history → |
| 34 | The HorseCliff Nobles & Co. | 54 | Chart history → |
| 35 | My Girl/Hey GirlBobby Vee | 35 | Chart history → |
| 36 | Young GirlThe Union Gap Featuring Gary Puckett | 17 | Chart history → |
| 37 | (You Keep Me) Hangin' OnJoe Simon | 41 | Chart history → |
| 38 | Never Give You UpJerry Butler | 50 | Chart history → |
| 39 | Choo Choo TrainThe Box Tops | 62 | Chart history → |
| 40 | Does Your Mama Know About MeBobby Taylor & The Vancouvers | 40 | Chart history → |
| 41 | Time For Livin'The Association | 45 | Chart history → |
| 42 | I'm SorryThe Delfonics | 42 | Chart history → |
| 43 | She's A HeartbreakerGene Pitney | 48 | Chart history → |
| 44 | I Wanna LiveGlen Campbell | 36 | Chart history → |
| 45 | The UnicornThe Irish Rovers | 18 | Chart history → |
| 46 | Cry Like A BabyThe Box Tops | 27 | Chart history → |
| 47 | Yester LoveSmokey Robinson & The Miracles | 73 | Chart history → |
| 48 | UnitedPeaches & Herb | 56 | Chart history → |
| 49 | If You Don't Want My LoveRobert John | 53 | Chart history → |
| 50 | Here Comes The JudgeShorty Long | 83 | Chart history → |
| 51 | Jelly Jungle (Of Orange Marmalade)Lemon Pipers | 51 | Chart history → |
| 52 | Indian LakeThe Cowsills | 79 | Chart history → |
| 53 | Stoned Soul PicnicThe 5th Dimension | 95 | Chart history → |
| 54 | Sky Pilot (Part One)Eric Burdon & The Animals | 86 | Chart history → |
| 55 | You Don't Know What You Mean To MeSam & Dave | 57 | Chart history → |
| 56 | UnwindRay Stevens | 52 | Chart history → |
| 57 | Bring A Little Lovin'Los Bravos | 75 | Chart history → |
| 58 | Brooklyn RoadsNeil Diamond | 58 | Chart history → |
| 59 | I'll Never Do You WrongJoe Tex | 61 | Chart history → |
| 60 | Love In Every RoomPaul Mauriat And His Orchestra | 60 | Chart history → |
| 61 | Sleepy JoeHerman's Hermits | 65 | Chart history → |
| 62 | Jumpin' Jack FlashThe Rolling Stones | — | Chart history → |
| 63 | Some Things You Never Get Used ToDiana Ross & The Supremes | — | Chart history → |
| 64 | Lady WillpowerGary Puckett And The Union Gap | — | Chart history → |
| 65 | Here Come The JudgeThe Magistrates | 100 | Chart history → |
| 66 | It Should Have Been MeGladys Knight And The Pips | — | Chart history → |
| 67 | May I Take A Giant Step (Into Your Heart)1910 Fruitgum Co. | 63 | Chart history → |
| 68 | I Wish I Knew (How It Would Feel To Be Free)Solomon Burke | 74 | Chart history → |
| 69 | America Is My Home - Pt. 1James Brown And The Famous Flames | 72 | Chart history → |
| 70 | The DoctorMary Wells | 70 | Chart history → |
| 71 | I Got You BabeEtta James | 71 | Chart history → |
| 72 | Anyone For TennisCream | 64 | Chart history → |
| 73 | Pictures Of Matchstick MenThe Status Quo | 98 | Chart history → |
| 74 | You Ain't Going NowhereThe Byrds | 77 | Chart history → |
| 75 | Folsom Prison BluesJohnny Cash | 84 | Chart history → |
| 76 | My Shy VioletThe Mills Brothers | 80 | Chart history → |
| 77 | Face It Girl, It's OverNancy Wilson | 81 | Chart history → |
| 78 | Back In Love AgainThe Buckinghams | — | Chart history → |
| 79 | Safe In My GardenThe Mamas & The Papas | — | Chart history → |
| 80 | It's OverEddy Arnold | 88 | Chart history → |
| 81 | Mountain Of LoveRonnie Dove | — | Chart history → |
| 82 | ApologizeEd Ames | 82 | Chart history → |
| 83 | Grazing In The GrassHugh Masekela | — | Chart history → |
| 84 | Ready, Willing and AbleThe American Breed | 85 | Chart history → |
| 85 | Here I Am BabyThe Marvelettes | — | Chart history → |
| 86 | Eleanor RigbyRay Charles | — | Chart history → |
| 87 | Lover's HolidayPeggy Scott & Jo Jo Benson | — | Chart history → |
| 88 | Funky FeverClarence Carter | 96 | Chart history → |
| 89 | Ain't Nothin' But A House PartyThe Show Stoppers | 97 | Chart history → |
| 90 | Lili MarleneAl Martino | 87 | Chart history → |
| 91 | San Francisco Girls (Return of the Native)Fever Tree | 91 | Chart history → |
| 92 | Hold OnRadiants | 92 | Chart history → |
| 93 | Let Me Be LonelyDionne Warwick | — | Chart history → |
| 94 | Here Come Da JudgeThe Buena Vistas | 94 | Chart history → |
| 95 | Baby You Come Rollin' Across My MindThe Peppermint Trolley Company | — | Chart history → |
| 96 | Sweet MemoriesAndy Williams | — | Chart history → |
| 97 | Climb Every MountainThe Hesitations | 90 | Chart history → |
| 98 | Don't Sign The Paper Baby (I Want You Back)Jimmy Delphs | 99 | Chart history → |
| 99 | Lonely Is The NameSammy Davis Jr. | 93 | Chart history → |
| 100 | CongratulationsCliff Richard | — | Chart history → |