| 1 | Mrs. RobinsonSimon & Garfunkel | 1 | Chart history → |
| 2 | This Guy's In Love With YouHerb Alpert | 3 | Chart history → |
| 3 | Mony MonyTommy James And The Shondells | 5 | Chart history → |
| 4 | Yummy Yummy YummyOhio Express | 6 | Chart history → |
| 5 | MacArthur ParkRichard Harris | 7 | Chart history → |
| 6 | Tighten UpArchie Bell & The Drells | 2 | Chart history → |
| 7 | ThinkAretha Franklin | 9 | Chart history → |
| 8 | A Beautiful MorningThe Rascals | 8 | Chart history → |
| 9 | The Good, The Bad And The UglyHugo Montenegro, His Orchestra And Chorus | 4 | Chart history → |
| 10 | The Look Of LoveSergio Mendes & Brasil '66 | 13 | Chart history → |
| 11 | Ain't Nothing Like The Real ThingMarvin Gaye & Tammi Terrell | 11 | Chart history → |
| 12 | HoneyBobby Goldsboro | 10 | Chart history → |
| 13 | I Could Never Love Another (After Loving You)The Temptations | 19 | Chart history → |
| 14 | Angel Of The MorningMerrilee Rush & The Turnabouts | 14 | Chart history → |
| 15 | The HorseCliff Nobles & Co. | 34 | Chart history → |
| 16 | DelilahTom Jones | 15 | Chart history → |
| 17 | Licking Stick - Licking Stick (Part 1)James Brown And The Famous Flames | 25 | Chart history → |
| 18 | I Love YouPeople | 22 | Chart history → |
| 19 | Here Comes The JudgeShorty Long | 50 | Chart history → |
| 20 | If I Were A CarpenterFour Tops | 20 | Chart history → |
| 21 | Do You Know The Way To San JoséDionne Warwick | 21 | Chart history → |
| 22 | Reach Out Of The DarknessFriend And Lover | 23 | Chart history → |
| 23 | Master JackFour Jacks And A Jill | 18 | Chart history → |
| 24 | Like To Get To Know YouSpanky And Our Gang | 17 | Chart history → |
| 25 | (You Keep Me) Hangin' OnJoe Simon | 37 | Chart history → |
| 26 | A Man Without Love (Quando M'innamoro)Engelbert Humperdinck | 27 | Chart history → |
| 27 | How'd We Ever Get This WayAndy Kim | 29 | Chart history → |
| 28 | Shoo-Be-Doo-Be-Doo-Da-DayStevie Wonder | 16 | Chart history → |
| 29 | Cowboys To GirlsThe Intruders | 12 | Chart history → |
| 30 | Tip-Toe Thru' The Tulips With MeTiny Tim | 33 | Chart history → |
| 31 | She's Lookin' GoodWilson Pickett | 30 | Chart history → |
| 32 | I Will Always Think About YouThe New Colony Six | 26 | Chart history → |
| 33 | Soul SerenadeWillie Mitchell | 32 | Chart history → |
| 34 | Choo Choo TrainThe Box Tops | 39 | Chart history → |
| 35 | Never Give You UpJerry Butler | 38 | Chart history → |
| 36 | Does Your Mama Know About MeBobby Taylor & The Vancouvers | 40 | Chart history → |
| 37 | Take Time To Know HerPercy Sledge | 24 | Chart history → |
| 38 | Jumpin' Jack FlashThe Rolling Stones | 62 | Chart history → |
| 39 | She's A HeartbreakerGene Pitney | 43 | Chart history → |
| 40 | Face It Girl, It's OverNancy Wilson | 77 | Chart history → |
| 41 | Time For Livin'The Association | 41 | Chart history → |
| 42 | I'm SorryThe Delfonics | 42 | Chart history → |
| 43 | The Happy Song (Dum-Dum)Otis Redding | 28 | Chart history → |
| 44 | I Wanna LiveGlen Campbell | 44 | Chart history → |
| 45 | Lady WillpowerGary Puckett And The Union Gap | 64 | Chart history → |
| 46 | UnitedPeaches & Herb | 48 | Chart history → |
| 47 | Yester LoveSmokey Robinson & The Miracles | 47 | Chart history → |
| 48 | You Don't Know What You Mean To MeSam & Dave | 55 | Chart history → |
| 49 | If You Don't Want My LoveRobert John | 49 | Chart history → |
| 50 | It Should Have Been MeGladys Knight And The Pips | 66 | Chart history → |
| 51 | Indian LakeThe Cowsills | 52 | Chart history → |
| 52 | Grazing In The GrassHugh Masekela | 83 | Chart history → |
| 53 | Stoned Soul PicnicThe 5th Dimension | 53 | Chart history → |
| 54 | Sky Pilot (Part One)Eric Burdon & The Animals | 54 | Chart history → |
| 55 | Folsom Prison BluesJohnny Cash | 75 | Chart history → |
| 56 | Some Things You Never Get Used ToDiana Ross & The Supremes | 63 | Chart history → |
| 57 | Bring A Little Lovin'Los Bravos | 57 | Chart history → |
| 58 | Pictures Of Matchstick MenThe Status Quo | 73 | Chart history → |
| 59 | I'll Never Do You WrongJoe Tex | 59 | Chart history → |
| 60 | Lover's HolidayPeggy Scott & Jo Jo Benson | 87 | Chart history → |
| 61 | D. W. WashburnThe Monkees | — | Chart history → |
| 62 | Here Come The JudgeThe Magistrates | 65 | Chart history → |
| 63 | My Girl/Hey GirlBobby Vee | 35 | Chart history → |
| 64 | America Is My Home - Pt. 1James Brown And The Famous Flames | 69 | Chart history → |
| 65 | Jelly Jungle (Of Orange Marmalade)Lemon Pipers | 51 | Chart history → |
| 66 | UnwindRay Stevens | 56 | Chart history → |
| 67 | Brooklyn RoadsNeil Diamond | 58 | Chart history → |
| 68 | I Wish I Knew (How It Would Feel To Be Free)Solomon Burke | 68 | Chart history → |
| 69 | I Got You BabeEtta James | 71 | Chart history → |
| 70 | The DoctorMary Wells | 70 | Chart history → |
| 71 | Eleanor RigbyRay Charles | 86 | Chart history → |
| 72 | Here I Am BabyThe Marvelettes | 85 | Chart history → |
| 73 | My Shy VioletThe Mills Brothers | 76 | Chart history → |
| 74 | It's OverEddy Arnold | 80 | Chart history → |
| 75 | Mountain Of LoveRonnie Dove | 81 | Chart history → |
| 76 | Back In Love AgainThe Buckinghams | 78 | Chart history → |
| 77 | Love In Every RoomPaul Mauriat And His Orchestra | 60 | Chart history → |
| 78 | Safe In My GardenThe Mamas & The Papas | 79 | Chart history → |
| 79 | ApologizeEd Ames | 82 | Chart history → |
| 80 | Sleepy JoeHerman's Hermits | 61 | Chart history → |
| 81 | You Send MeAretha Franklin | — | Chart history → |
| 82 | Here Comes The JudgePigmeat Markham | — | Chart history → |
| 83 | Let Me Be LonelyDionne Warwick | 93 | Chart history → |
| 84 | It's Nice To Be With YouThe Monkees | — | Chart history → |
| 85 | Sweet MemoriesAndy Williams | 96 | Chart history → |
| 86 | Hold OnRadiants | 92 | Chart history → |
| 87 | UnderstandingRay Charles | — | Chart history → |
| 88 | Funky FeverClarence Carter | 88 | Chart history → |
| 89 | Ain't Nothin' But A House PartyThe Show Stoppers | 89 | Chart history → |
| 90 | Can't You See Me CryThe New Colony Six | — | Chart history → |
| 91 | San Francisco Girls (Return of the Native)Fever Tree | 91 | Chart history → |
| 92 | Baby You Come Rollin' Across My MindThe Peppermint Trolley Company | 95 | Chart history → |
| 93 | Here Come Da JudgeThe Buena Vistas | 94 | Chart history → |
| 94 | Let Yourself GoElvis Presley With The Jordanaires | — | Chart history → |
| 95 | Turn Around, Look At MeThe Vogues | — | Chart history → |
| 96 | Don't Sign The Paper Baby (I Want You Back)Jimmy Delphs | 98 | Chart history → |
| 97 | Listen HereEddie Harris | — | Chart history → |
| 98 | Forget Me NotMartha Reeves & The Vandellas | — | Chart history → |
| 99 | Valley Of The DollsKing Curtis & The Kingpins | — | Chart history → |
| 100 | CongratulationsCliff Richard | 100 | Chart history → |