| 1 | This Guy's In Love With YouHerb Alpert | 1 | Chart history → |
| 2 | The HorseCliff Nobles & Co. | 2 | Chart history → |
| 3 | Jumpin' Jack FlashThe Rolling Stones | 3 | Chart history → |
| 4 | Lady WillpowerGary Puckett And The Union Gap | 6 | Chart history → |
| 5 | Grazing In The GrassHugh Masekela | 5 | Chart history → |
| 6 | The Look Of LoveSergio Mendes & Brasil '66 | 4 | Chart history → |
| 7 | Angel Of The MorningMerrilee Rush & The Turnabouts | 7 | Chart history → |
| 8 | Stoned Soul PicnicThe 5th Dimension | 17 | Chart history → |
| 9 | Here Comes The JudgeShorty Long | 8 | Chart history → |
| 10 | Indian LakeThe Cowsills | 15 | Chart history → |
| 11 | Reach Out Of The DarknessFriend And Lover | 10 | Chart history → |
| 12 | Hurdy Gurdy ManDonovan | 23 | Chart history → |
| 13 | Mony MonyTommy James And The Shondells | 12 | Chart history → |
| 14 | MacArthur ParkRichard Harris | 9 | Chart history → |
| 15 | Yummy Yummy YummyOhio Express | 11 | Chart history → |
| 16 | Mrs. RobinsonSimon & Garfunkel | 13 | Chart history → |
| 17 | I Love YouPeople | 16 | Chart history → |
| 18 | ThinkAretha Franklin | 14 | Chart history → |
| 19 | D. W. WashburnThe Monkees | 19 | Chart history → |
| 20 | She's A HeartbreakerGene Pitney | 22 | Chart history → |
| 21 | Turn Around, Look At MeThe Vogues | 43 | Chart history → |
| 22 | Hello, I Love YouThe Doors | 77 | Chart history → |
| 23 | Never Give You UpJerry Butler | 20 | Chart history → |
| 24 | Here Comes The JudgePigmeat Markham | 24 | Chart history → |
| 25 | (You Keep Me) Hangin' OnJoe Simon | 25 | Chart history → |
| 26 | Choo Choo TrainThe Box Tops | 26 | Chart history → |
| 27 | Pictures Of Matchstick MenThe Status Quo | 34 | Chart history → |
| 28 | Sky Pilot (Part One)Eric Burdon & The Animals | 29 | Chart history → |
| 29 | Classical GasMason Williams | 55 | Chart history → |
| 30 | Some Things You Never Get Used ToDiana Ross & The Supremes | 30 | Chart history → |
| 31 | How'd We Ever Get This WayAndy Kim | 21 | Chart history → |
| 32 | Folsom Prison BluesJohnny Cash | 32 | Chart history → |
| 33 | Licking Stick - Licking Stick (Part 1)James Brown And The Famous Flames | 18 | Chart history → |
| 34 | Tip-Toe Thru' The Tulips With MeTiny Tim | 27 | Chart history → |
| 35 | Autumn Of My LifeBobby Goldsboro | 44 | Chart history → |
| 36 | I'm A Midnight MoverWilson Pickett | 37 | Chart history → |
| 37 | Face It Girl, It's OverNancy Wilson | 38 | Chart history → |
| 38 | Don't Take It So HardPaul Revere & The Raiders Featuring Mark Lindsay | 42 | Chart history → |
| 39 | Lover's HolidayPeggy Scott & Jo Jo Benson | 39 | Chart history → |
| 40 | Yester LoveSmokey Robinson & The Miracles | 31 | Chart history → |
| 41 | Sunshine Of Your LoveCream | 52 | Chart history → |
| 42 | It Should Have Been MeGladys Knight And The Pips | 40 | Chart history → |
| 43 | The Good, The Bad And The UglyHugo Montenegro, His Orchestra And Chorus | 28 | Chart history → |
| 44 | Eleanor RigbyRay Charles | 45 | Chart history → |
| 45 | Dreams Of The Everyday HousewifeGlen Campbell | 73 | Chart history → |
| 46 | Sealed With A KissGary Lewis And The Playboys | 79 | Chart history → |
| 47 | Stay In My CornerThe Dells | 47 | Chart history → |
| 48 | The Story Of Rock And RollThe Turtles | 63 | Chart history → |
| 49 | Here I Am BabyThe Marvelettes | 49 | Chart history → |
| 50 | Journey To The Center Of The MindThe Amboy Dukes | 64 | Chart history → |
| 51 | It's Nice To Be With YouThe Monkees | 51 | Chart history → |
| 52 | You Don't Know What You Mean To MeSam & Dave | 48 | Chart history → |
| 53 | Dream A Little Dream Of MeMama Cass With The Mamas & The Papas | 94 | Chart history → |
| 54 | Can't You See Me CryThe New Colony Six | 62 | Chart history → |
| 55 | The Eyes Of A New York WomanB.J. Thomas | 85 | Chart history → |
| 56 | You Send MeAretha Franklin | 61 | Chart history → |
| 57 | Hitch It To The HorseThe Fantastic Johnny C | 72 | Chart history → |
| 58 | People Sure Act FunnyArthur Conley | 58 | Chart history → |
| 59 | Safe In My GardenThe Mamas & The Papas | 53 | Chart history → |
| 60 | Baby You Come Rollin' Across My MindThe Peppermint Trolley Company | 65 | Chart history → |
| 61 | Here Come The JudgeThe Magistrates | 54 | Chart history → |
| 62 | AmenOtis Redding | 91 | Chart history → |
| 63 | With Pen In HandBilly Vera | 70 | Chart history → |
| 64 | D-I-V-O-R-C-ETammy Wynette | 76 | Chart history → |
| 65 | Be Young, Be Foolish, Be HappyThe Tams | 66 | Chart history → |
| 66 | Alice Long (You're Still My Favorite Girlfriend)Tommy Boyce & Bobby Hart | 88 | Chart history → |
| 67 | Mountain Of LoveRonnie Dove | 67 | Chart history → |
| 68 | Back In Love AgainThe Buckinghams | 57 | Chart history → |
| 69 | UnderstandingRay Charles | 69 | Chart history → |
| 70 | Born To Be WildSteppenwolf | — | Chart history → |
| 71 | Let Yourself GoElvis Presley With The Jordanaires | 81 | Chart history → |
| 72 | Your Time Hasn't Come Yet, BabyElvis Presley With The Jordanaires | 82 | Chart history → |
| 73 | You Keep Me Hangin' OnThe Vanilla Fudge | — | Chart history → |
| 74 | Hold OnRadiants | 74 | Chart history → |
| 75 | (The Puppet Song) Whiskey On A SundayThe Irish Rovers | 80 | Chart history → |
| 76 | Dreams Of The Everyday HousewifeWayne Newton | 89 | Chart history → |
| 77 | The Impossible DreamRoger Williams | — | Chart history → |
| 78 | (Love Is Like A) Baseball GameThe Intruders | 99 | Chart history → |
| 79 | Sweet MemoriesAndy Williams | 75 | Chart history → |
| 80 | Listen HereEddie Harris | 78 | Chart history → |
| 81 | Lovin' SeasonGene And Debbe | 84 | Chart history → |
| 82 | Hang 'Em HighHugo Montenegro, His Orchestra And Chorus | 86 | Chart history → |
| 83 | Turn On Your Love LightBill Black's Combo | 83 | Chart history → |
| 84 | Soul-LimboBooker T. & The MG's | — | Chart history → |
| 85 | Competition Ain't Nothin'Little Carl Carlton | 96 | Chart history → |
| 86 | Prayer Meetin'Willie Mitchell | — | Chart history → |
| 87 | Young BoyBarbara Greene | 87 | Chart history → |
| 88 | Hard To HandleOtis Redding | — | Chart history → |
| 89 | Snoopy For PresidentThe Royal Guardsmen | — | Chart history → |
| 90 | Look Over Your ShoulderThe O'Jays | 90 | Chart history → |
| 91 | To Love SomebodyThe Sweet Inspirations | 93 | Chart history → |
| 92 | Georgia On My MindWes Montgomery | 92 | Chart history → |
| 93 | Just A Little BitBlue Cheer | 97 | Chart history → |
| 94 | Mrs. BluebirdEternity's Children | — | Chart history → |
| 95 | What's Made Milwaukee Famous (Has Made A Loser Out Of Me)Jerry Lee Lewis | 95 | Chart history → |
| 96 | Little Green ApplesPatti Page | 98 | Chart history → |
| 97 | Slip AwayClarence Carter | — | Chart history → |
| 98 | Love Makes A WomanBarbara Acklin | — | Chart history → |
| 99 | Two-Bit ManchildNeil Diamond | — | Chart history → |
| 100 | Send My Baby BackFreddie Hughes | 100 | Chart history → |