| 1 | Grazing In The GrassHugh Masekela | 5 | Chart history → |
| 2 | Lady WillpowerGary Puckett And The Union Gap | 4 | Chart history → |
| 3 | Jumpin' Jack FlashThe Rolling Stones | 3 | Chart history → |
| 4 | This Guy's In Love With YouHerb Alpert | 1 | Chart history → |
| 5 | The HorseCliff Nobles & Co. | 2 | Chart history → |
| 6 | Stoned Soul PicnicThe 5th Dimension | 8 | Chart history → |
| 7 | Hurdy Gurdy ManDonovan | 12 | Chart history → |
| 8 | Classical GasMason Williams | 29 | Chart history → |
| 9 | Hello, I Love YouThe Doors | 22 | Chart history → |
| 10 | Indian LakeThe Cowsills | 10 | Chart history → |
| 11 | Reach Out Of The DarknessFriend And Lover | 11 | Chart history → |
| 12 | Here Comes The JudgeShorty Long | 9 | Chart history → |
| 13 | Angel Of The MorningMerrilee Rush & The Turnabouts | 7 | Chart history → |
| 14 | Turn Around, Look At MeThe Vogues | 21 | Chart history → |
| 15 | The Look Of LoveSergio Mendes & Brasil '66 | 6 | Chart history → |
| 16 | She's A HeartbreakerGene Pitney | 20 | Chart history → |
| 17 | MacArthur ParkRichard Harris | 14 | Chart history → |
| 18 | Yummy Yummy YummyOhio Express | 15 | Chart history → |
| 19 | I Love YouPeople | 17 | Chart history → |
| 20 | Sky Pilot (Part One)Eric Burdon & The Animals | 28 | Chart history → |
| 21 | Pictures Of Matchstick MenThe Status Quo | 27 | Chart history → |
| 22 | Sunshine Of Your LoveCream | 41 | Chart history → |
| 23 | Here Comes The JudgePigmeat Markham | 24 | Chart history → |
| 24 | Mony MonyTommy James And The Shondells | 13 | Chart history → |
| 25 | Never Give You UpJerry Butler | 23 | Chart history → |
| 26 | Autumn Of My LifeBobby Goldsboro | 35 | Chart history → |
| 27 | ThinkAretha Franklin | 18 | Chart history → |
| 28 | I'm A Midnight MoverWilson Pickett | 36 | Chart history → |
| 29 | Mrs. RobinsonSimon & Garfunkel | 16 | Chart history → |
| 30 | Some Things You Never Get Used ToDiana Ross & The Supremes | 30 | Chart history → |
| 31 | D. W. WashburnThe Monkees | 19 | Chart history → |
| 32 | Folsom Prison BluesJohnny Cash | 32 | Chart history → |
| 33 | Lover's HolidayPeggy Scott & Jo Jo Benson | 39 | Chart history → |
| 34 | Don't Take It So HardPaul Revere & The Raiders Featuring Mark Lindsay | 38 | Chart history → |
| 35 | (You Keep Me) Hangin' OnJoe Simon | 25 | Chart history → |
| 36 | Stay In My CornerThe Dells | 47 | Chart history → |
| 37 | Face It Girl, It's OverNancy Wilson | 37 | Chart history → |
| 38 | How'd We Ever Get This WayAndy Kim | 31 | Chart history → |
| 39 | Born To Be WildSteppenwolf | 70 | Chart history → |
| 40 | Eleanor RigbyRay Charles | 44 | Chart history → |
| 41 | Dream A Little Dream Of MeMama Cass With The Mamas & The Papas | 53 | Chart history → |
| 42 | Choo Choo TrainThe Box Tops | 26 | Chart history → |
| 43 | With Pen In HandBilly Vera | 63 | Chart history → |
| 44 | AmenOtis Redding | 62 | Chart history → |
| 45 | Dreams Of The Everyday HousewifeGlen Campbell | 45 | Chart history → |
| 46 | Sealed With A KissGary Lewis And The Playboys | 46 | Chart history → |
| 47 | Journey To The Center Of The MindThe Amboy Dukes | 50 | Chart history → |
| 48 | The Story Of Rock And RollThe Turtles | 48 | Chart history → |
| 49 | Here I Am BabyThe Marvelettes | 49 | Chart history → |
| 50 | It Should Have Been MeGladys Knight And The Pips | 42 | Chart history → |
| 51 | It's Nice To Be With YouThe Monkees | 51 | Chart history → |
| 52 | Soul-LimboBooker T. & The MG's | 84 | Chart history → |
| 53 | Hitch It To The HorseThe Fantastic Johnny C | 57 | Chart history → |
| 54 | Can't You See Me CryThe New Colony Six | 54 | Chart history → |
| 55 | The Eyes Of A New York WomanB.J. Thomas | 55 | Chart history → |
| 56 | You Keep Me Hangin' OnThe Vanilla Fudge | 73 | Chart history → |
| 57 | Yester LoveSmokey Robinson & The Miracles | 40 | Chart history → |
| 58 | People Sure Act FunnyArthur Conley | 58 | Chart history → |
| 59 | Alice Long (You're Still My Favorite Girlfriend)Tommy Boyce & Bobby Hart | 66 | Chart history → |
| 60 | Baby You Come Rollin' Across My MindThe Peppermint Trolley Company | 60 | Chart history → |
| 61 | Be Young, Be Foolish, Be HappyThe Tams | 65 | Chart history → |
| 62 | Prayer Meetin'Willie Mitchell | 86 | Chart history → |
| 63 | D-I-V-O-R-C-ETammy Wynette | 64 | Chart history → |
| 64 | People Got To Be FreeThe Rascals | — | Chart history → |
| 65 | Halfway To ParadiseBobby Vinton | — | Chart history → |
| 66 | UnderstandingRay Charles | 69 | Chart history → |
| 67 | You Send MeAretha Franklin | 56 | Chart history → |
| 68 | Hold OnRadiants | 74 | Chart history → |
| 69 | The Impossible DreamRoger Williams | 77 | Chart history → |
| 70 | (Love Is Like A) Baseball GameThe Intruders | 78 | Chart history → |
| 71 | Love Makes A WomanBarbara Acklin | 98 | Chart history → |
| 72 | Your Time Hasn't Come Yet, BabyElvis Presley With The Jordanaires | 72 | Chart history → |
| 73 | You Met Your MatchStevie Wonder | — | Chart history → |
| 74 | To Love SomebodyThe Sweet Inspirations | 91 | Chart history → |
| 75 | (The Puppet Song) Whiskey On A SundayThe Irish Rovers | 75 | Chart history → |
| 76 | Dreams Of The Everyday HousewifeWayne Newton | 76 | Chart history → |
| 77 | Two-Bit ManchildNeil Diamond | 99 | Chart history → |
| 78 | I Can't Stop DancingArchie Bell & The Drells | — | Chart history → |
| 79 | Hard To HandleOtis Redding | 88 | Chart history → |
| 80 | Mrs. BluebirdEternity's Children | 94 | Chart history → |
| 81 | Lovin' SeasonGene And Debbe | 81 | Chart history → |
| 82 | Hang 'Em HighHugo Montenegro, His Orchestra And Chorus | 82 | Chart history → |
| 83 | Turn On Your Love LightBill Black's Combo | 83 | Chart history → |
| 84 | Competition Ain't Nothin'Little Carl Carlton | 85 | Chart history → |
| 85 | Snoopy For PresidentThe Royal Guardsmen | 89 | Chart history → |
| 86 | Young BoyBarbara Greene | 87 | Chart history → |
| 87 | God Bless Our LoveThe Ballads | — | Chart history → |
| 88 | Don't Give UpPetula Clark | — | Chart history → |
| 89 | Look Over Your ShoulderThe O'Jays | 90 | Chart history → |
| 90 | I Get The Sweetest FeelingJackie Wilson | — | Chart history → |
| 91 | Georgia On My MindWes Montgomery | 92 | Chart history → |
| 92 | Just A Little BitBlue Cheer | 93 | Chart history → |
| 93 | Slip AwayClarence Carter | 97 | Chart history → |
| 94 | What's Made Milwaukee Famous (Has Made A Loser Out Of Me)Jerry Lee Lewis | 95 | Chart history → |
| 95 | And SuddenlyThe Cherry People | — | Chart history → |
| 96 | Yesterday's DreamsFour Tops | — | Chart history → |
| 97 | I Loved And I LostThe Impressions | — | Chart history → |
| 98 | Tuesday Afternoon (Forever Afternoon)The Moody Blues | — | Chart history → |
| 99 | Send My Baby BackFreddie Hughes | 100 | Chart history → |
| 100 | Give Me One More ChanceWilmer And The Dukes | — | Chart history → |