| 1 | Grazing In The GrassHugh Masekela | 1 | Chart history → |
| 2 | Lady WillpowerGary Puckett And The Union Gap | 2 | Chart history → |
| 3 | Stoned Soul PicnicThe 5th Dimension | 6 | Chart history → |
| 4 | Jumpin' Jack FlashThe Rolling Stones | 3 | Chart history → |
| 5 | The HorseCliff Nobles & Co. | 5 | Chart history → |
| 6 | Hurdy Gurdy ManDonovan | 7 | Chart history → |
| 7 | This Guy's In Love With YouHerb Alpert | 4 | Chart history → |
| 8 | Classical GasMason Williams | 8 | Chart history → |
| 9 | Hello, I Love YouThe Doors | 9 | Chart history → |
| 10 | Indian LakeThe Cowsills | 10 | Chart history → |
| 11 | Turn Around, Look At MeThe Vogues | 14 | Chart history → |
| 12 | Here Comes The JudgeShorty Long | 12 | Chart history → |
| 13 | Reach Out Of The DarknessFriend And Lover | 11 | Chart history → |
| 14 | Sky Pilot (Part One)Eric Burdon & The Animals | 20 | Chart history → |
| 15 | Pictures Of Matchstick MenThe Status Quo | 21 | Chart history → |
| 16 | The Look Of LoveSergio Mendes & Brasil '66 | 15 | Chart history → |
| 17 | Angel Of The MorningMerrilee Rush & The Turnabouts | 13 | Chart history → |
| 18 | Sunshine Of Your LoveCream | 22 | Chart history → |
| 19 | Here Comes The JudgePigmeat Markham | 23 | Chart history → |
| 20 | She's A HeartbreakerGene Pitney | 16 | Chart history → |
| 21 | Autumn Of My LifeBobby Goldsboro | 26 | Chart history → |
| 22 | I Love YouPeople | 19 | Chart history → |
| 23 | MacArthur ParkRichard Harris | 17 | Chart history → |
| 24 | I'm A Midnight MoverWilson Pickett | 28 | Chart history → |
| 25 | Stay In My CornerThe Dells | 36 | Chart history → |
| 26 | Never Give You UpJerry Butler | 25 | Chart history → |
| 27 | Don't Take It So HardPaul Revere & The Raiders Featuring Mark Lindsay | 34 | Chart history → |
| 28 | Yummy Yummy YummyOhio Express | 18 | Chart history → |
| 29 | Face It Girl, It's OverNancy Wilson | 37 | Chart history → |
| 30 | Dream A Little Dream Of MeMama Cass With The Mamas & The Papas | 41 | Chart history → |
| 31 | Born To Be WildSteppenwolf | 39 | Chart history → |
| 32 | People Got To Be FreeThe Rascals | 64 | Chart history → |
| 33 | Lover's HolidayPeggy Scott & Jo Jo Benson | 33 | Chart history → |
| 34 | Mony MonyTommy James And The Shondells | 24 | Chart history → |
| 35 | Eleanor RigbyRay Charles | 40 | Chart history → |
| 36 | AmenOtis Redding | 44 | Chart history → |
| 37 | Folsom Prison BluesJohnny Cash | 32 | Chart history → |
| 38 | Journey To The Center Of The MindThe Amboy Dukes | 47 | Chart history → |
| 39 | D. W. WashburnThe Monkees | 31 | Chart history → |
| 40 | Sealed With A KissGary Lewis And The Playboys | 46 | Chart history → |
| 41 | Hitch It To The HorseThe Fantastic Johnny C | 53 | Chart history → |
| 42 | Soul-LimboBooker T. & The MG's | 52 | Chart history → |
| 43 | With Pen In HandBilly Vera | 43 | Chart history → |
| 44 | Here I Am BabyThe Marvelettes | 49 | Chart history → |
| 45 | Dreams Of The Everyday HousewifeGlen Campbell | 45 | Chart history → |
| 46 | The Eyes Of A New York WomanB.J. Thomas | 55 | Chart history → |
| 47 | You Keep Me Hangin' OnThe Vanilla Fudge | 56 | Chart history → |
| 48 | You Met Your MatchStevie Wonder | 73 | Chart history → |
| 49 | I Can't Stop DancingArchie Bell & The Drells | 78 | Chart history → |
| 50 | It Should Have Been MeGladys Knight And The Pips | 50 | Chart history → |
| 51 | It's Nice To Be With YouThe Monkees | 51 | Chart history → |
| 52 | Can't You See Me CryThe New Colony Six | 54 | Chart history → |
| 53 | Halfway To ParadiseBobby Vinton | 65 | Chart history → |
| 54 | Yesterday's DreamsFour Tops | 96 | Chart history → |
| 55 | The Story Of Rock And RollThe Turtles | 48 | Chart history → |
| 56 | Alice Long (You're Still My Favorite Girlfriend)Tommy Boyce & Bobby Hart | 59 | Chart history → |
| 57 | (Love Is Like A) Baseball GameThe Intruders | 70 | Chart history → |
| 58 | Love Makes A WomanBarbara Acklin | 71 | Chart history → |
| 59 | Baby You Come Rollin' Across My MindThe Peppermint Trolley Company | 60 | Chart history → |
| 60 | Prayer Meetin'Willie Mitchell | 62 | Chart history → |
| 61 | Be Young, Be Foolish, Be HappyThe Tams | 61 | Chart history → |
| 62 | Light My FireJose Feliciano | — | Chart history → |
| 63 | Hard To HandleOtis Redding | 79 | Chart history → |
| 64 | The Impossible DreamRoger Williams | 69 | Chart history → |
| 65 | UnderstandingRay Charles | 66 | Chart history → |
| 66 | I Get The Sweetest FeelingJackie Wilson | 90 | Chart history → |
| 67 | Slip AwayClarence Carter | 93 | Chart history → |
| 68 | Dreams Of The Everyday HousewifeWayne Newton | 76 | Chart history → |
| 69 | D-I-V-O-R-C-ETammy Wynette | 63 | Chart history → |
| 70 | Two-Bit ManchildNeil Diamond | 77 | Chart history → |
| 71 | Tuesday Afternoon (Forever Afternoon)The Moody Blues | 98 | Chart history → |
| 72 | Your Time Hasn't Come Yet, BabyElvis Presley With The Jordanaires | 72 | Chart history → |
| 73 | Mrs. BluebirdEternity's Children | 80 | Chart history → |
| 74 | To Love SomebodyThe Sweet Inspirations | 74 | Chart history → |
| 75 | (The Puppet Song) Whiskey On A SundayThe Irish Rovers | 75 | Chart history → |
| 76 | Competition Ain't Nothin'Little Carl Carlton | 84 | Chart history → |
| 77 | I Guess I'll Have To Cry, Cry, CryJames Brown And The Famous Flames | — | Chart history → |
| 78 | Don't Give UpPetula Clark | 88 | Chart history → |
| 79 | HappyNancy Sinatra | — | Chart history → |
| 80 | You're All I Need To Get ByMarvin Gaye & Tammi Terrell | — | Chart history → |
| 81 | And SuddenlyThe Cherry People | 95 | Chart history → |
| 82 | Turn On Your Love LightBill Black's Combo | 83 | Chart history → |
| 83 | Hang 'Em HighHugo Montenegro, His Orchestra And Chorus | 82 | Chart history → |
| 84 | 1, 2, 3, Red Light1910 Fruitgum Co. | — | Chart history → |
| 85 | God Bless Our LoveThe Ballads | 87 | Chart history → |
| 86 | Breaking Up Is Hard To DoThe Happenings | — | Chart history → |
| 87 | Young BoyBarbara Greene | 86 | Chart history → |
| 88 | Do It AgainThe Beach Boys | — | Chart history → |
| 89 | Look Over Your ShoulderThe O'Jays | 89 | Chart history → |
| 90 | Somebody CaresTommy James And The Shondells | — | Chart history → |
| 91 | I've Never Found A Girl (To Love Me Like You Do)Eddie Floyd | — | Chart history → |
| 92 | Just A Little BitBlue Cheer | 92 | Chart history → |
| 93 | LifeSly & The Family Stone | — | Chart history → |
| 94 | I'm Gonna Do What They Do To MeB.B. King | — | Chart history → |
| 95 | I Loved And I LostThe Impressions | 97 | Chart history → |
| 96 | Mr. BojanglesJerry Jeff Walker | — | Chart history → |
| 97 | Send My Baby BackFreddie Hughes | 99 | Chart history → |
| 98 | Never Going BackThe Lovin' Spoonful | — | Chart history → |
| 99 | Soul MeetingThe Soul Clan | — | Chart history → |
| 100 | Give Me One More ChanceWilmer And The Dukes | 100 | Chart history → |