| 1 | I Heard It Through The GrapevineMarvin Gaye | 1 | Chart history → |
| 2 | For Once In My LifeStevie Wonder | 3 | Chart history → |
| 3 | Love ChildDiana Ross & The Supremes | 2 | Chart history → |
| 4 | Wichita LinemanGlen Campbell | 5 | Chart history → |
| 5 | StormyClassics IV Featuring Dennis Yost | 6 | Chart history → |
| 6 | Abraham, Martin And JohnDion | 4 | Chart history → |
| 7 | I'm Gonna Make You Love MeDiana Ross And The Supremes & The Temptations | 17 | Chart history → |
| 8 | Who's Making LoveJohnnie Taylor | 7 | Chart history → |
| 9 | I Love How You Love MeBobby Vinton | 9 | Chart history → |
| 10 | Cloud NineThe Temptations | 12 | Chart history → |
| 11 | Both Sides NowJudy Collins | 8 | Chart history → |
| 12 | CinnamonDerek | 13 | Chart history → |
| 13 | Hooked On A FeelingB.J. Thomas | 22 | Chart history → |
| 14 | See SawAretha Franklin | 14 | Chart history → |
| 15 | Hey JudeThe Beatles | 11 | Chart history → |
| 16 | Soulful StrutYoung-Holt Unlimited | 20 | Chart history → |
| 17 | Bring It On Home To MeEddie Floyd | 18 | Chart history → |
| 18 | Magic Carpet RideSteppenwolf | 10 | Chart history → |
| 19 | Chewy ChewyOhio Express | 15 | Chart history → |
| 20 | Going Up The CountryCanned Heat | 26 | Chart history → |
| 21 | Son-Of-A Preacher ManDusty Springfield | 24 | Chart history → |
| 22 | Little ArrowsLeapy Lee | 21 | Chart history → |
| 23 | Too Weak To FightClarence Carter | 28 | Chart history → |
| 24 | Papa's Got A Brand New BagOtis Redding | 31 | Chart history → |
| 25 | Those Were The DaysMary Hopkin | 19 | Chart history → |
| 26 | Lo Mucho Que Te Quiero (The More I Love You)Rene & Rene | 30 | Chart history → |
| 27 | Scarborough FairSergio Mendes & Brasil '66 | 16 | Chart history → |
| 28 | Crimson And CloverTommy James And The Shondells | 39 | Chart history → |
| 29 | Shame, ShameMagic Lanterns | 29 | Chart history → |
| 30 | If I Can DreamElvis Presley | 36 | Chart history → |
| 31 | TillThe Vogues | 27 | Chart history → |
| 32 | A Ray Of HopeThe Rascals | 35 | Chart history → |
| 33 | Battle Hymn Of The RepublicAndy Williams with the St. Charles Borromeo Choir | 34 | Chart history → |
| 34 | Stand By Your ManTammy Wynette | 51 | Chart history → |
| 35 | Promises, PromisesDionne Warwick | 23 | Chart history → |
| 36 | My SongAretha Franklin | 54 | Chart history → |
| 37 | I Can't Turn You LooseThe Chambers Brothers | 37 | Chart history → |
| 38 | This Is My CountryThe Impressions | 43 | Chart history → |
| 39 | PeopleThe Tymes | 53 | Chart history → |
| 40 | Hang 'Em HighBooker T. & The MG's | 41 | Chart history → |
| 41 | I Started A JokeBee Gees | 61 | Chart history → |
| 42 | Everyday PeopleSly & The Family Stone | 55 | Chart history → |
| 43 | Hey JudeWilson Pickett | 90 | Chart history → |
| 44 | Put Your Head On My ShoulderThe Lettermen | 46 | Chart history → |
| 45 | Kentucky WomanDeep Purple | 38 | Chart history → |
| 46 | Bella LindaThe Grass Roots | 49 | Chart history → |
| 47 | My Favorite ThingsHerb Alpert & The Tijuana Brass | 47 | Chart history → |
| 48 | Baby Let's WaitThe Royal Guardsmen | 50 | Chart history → |
| 49 | There's Gonna Be A ShowdownArchie Bell & The Drells | 75 | Chart history → |
| 50 | Ready Or Not Here I Come (Can't Hide From Love)The Delfonics | 60 | Chart history → |
| 51 | MalindaBobby Taylor & The Vancouvers | 57 | Chart history → |
| 52 | Not Enough IndiansDean Martin | 44 | Chart history → |
| 53 | Worst That Could HappenBrooklyn Bridge | 98 | Chart history → |
| 54 | Ballad Of Two BrothersAutry Inman | 48 | Chart history → |
| 55 | The Girl Most LikelyJeannie C. Riley | 56 | Chart history → |
| 56 | Crosstown TrafficThe Jimi Hendrix Experience | 52 | Chart history → |
| 57 | Are You HappyJerry Butler | 78 | Chart history → |
| 58 | I Put A Spell On YouCreedence Clearwater Revival | 59 | Chart history → |
| 59 | American BoysPetula Clark | 62 | Chart history → |
| 60 | Rockin' In The Same Old BoatBobby Bland | 64 | Chart history → |
| 61 | Bluebirds Over The MountainThe Beach Boys | 67 | Chart history → |
| 62 | California SoulThe 5th Dimension | 72 | Chart history → |
| 63 | Isn't It Lonely TogetherO.C. Smith | 76 | Chart history → |
| 64 | Daddy Sang BassJohnny Cash | — | Chart history → |
| 65 | Season Of The Witch, Pt. 1Vanilla Fudge | 73 | Chart history → |
| 66 | Can I Change My MindTyrone Davis | 74 | Chart history → |
| 67 | White HousesEric Burdon & The Animals | 68 | Chart history → |
| 68 | Just Ain't No LoveBarbara Acklin | 70 | Chart history → |
| 69 | California Dreamin'Bobby Womack | 71 | Chart history → |
| 70 | Soul Sister, Brown SugarSam & Dave | 81 | Chart history → |
| 71 | The Beginning Of My EndThe Unifics | 85 | Chart history → |
| 72 | Touch MeThe Doors | — | Chart history → |
| 73 | A Minute Of Your TimeTom Jones | 88 | Chart history → |
| 74 | I've Gotta Be MeSammy Davis Jr. | 93 | Chart history → |
| 75 | Ramblin' Gamblin' ManBob Seger System | 84 | Chart history → |
| 76 | Love MachineThe O'Kaysions | 77 | Chart history → |
| 77 | Good Time GirlNancy Sinatra | 65 | Chart history → |
| 78 | Chitty Chitty Bang BangPaul Mauriat | 83 | Chart history → |
| 79 | Reach OutMerrilee Rush | 82 | Chart history → |
| 80 | VanceRoger Miller | 97 | Chart history → |
| 81 | You Got SoulJohnny Nash | 89 | Chart history → |
| 82 | Release MeJohnny Adams | 86 | Chart history → |
| 83 | Electric StoriesThe 4 Seasons Featuring the "Sound of Frankie Valli" | — | Chart history → |
| 84 | Rainbow RideAndy Kim | 87 | Chart history → |
| 85 | Not On The OutsideThe Moments | — | Chart history → |
| 86 | Tit For Tat (Ain't No Taking Back)James Brown | 92 | Chart history → |
| 87 | KayJohn Wesley Ryles, I | — | Chart history → |
| 88 | Feelin' So Good (S.k.o.o.b.y-D.o.o)The Archies | — | Chart history → |
| 89 | Sweet Cream Ladies, Forward MarchThe Box Tops | — | Chart history → |
| 90 | This Magic MomentJay & The Americans | — | Chart history → |
| 91 | Stay Close To MeFive Stairsteps & Cubie | 95 | Chart history → |
| 92 | EloiseBarry Ryan | — | Chart history → |
| 93 | You've Got The PowerThe Esquires | — | Chart history → |
| 94 | Does Anybody Know I'm HereThe Dells | — | Chart history → |
| 95 | The Thought Of Loving YouThe Crystal Mansion | 99 | Chart history → |
| 96 | Shout! - Part 1Chambers Brothers | 96 | Chart history → |
| 97 | Condition RedThe Goodees | 100 | Chart history → |
| 98 | I'm Into Lookin' For Someone To Love MeBobby Vee | — | Chart history → |
| 99 | I Can't Help It (If I'm Still In Love With You)Al Martino | — | Chart history → |
| 100 | Things I'd Like To SayNew Colony Six | — | Chart history → |