| 1 | I Heard It Through The GrapevineMarvin Gaye | 1 | Chart history → |
| 2 | For Once In My LifeStevie Wonder | 2 | Chart history → |
| 3 | I'm Gonna Make You Love MeDiana Ross And The Supremes & The Temptations | 7 | Chart history → |
| 4 | Soulful StrutYoung-Holt Unlimited | 16 | Chart history → |
| 5 | Wichita LinemanGlen Campbell | 4 | Chart history → |
| 6 | Cloud NineThe Temptations | 10 | Chart history → |
| 7 | Love ChildDiana Ross & The Supremes | 3 | Chart history → |
| 8 | StormyClassics IV Featuring Dennis Yost | 5 | Chart history → |
| 9 | Who's Making LoveJohnnie Taylor | 8 | Chart history → |
| 10 | Hooked On A FeelingB.J. Thomas | 13 | Chart history → |
| 11 | I Love How You Love MeBobby Vinton | 9 | Chart history → |
| 12 | CinnamonDerek | 12 | Chart history → |
| 13 | Too Weak To FightClarence Carter | 23 | Chart history → |
| 14 | Lo Mucho Que Te Quiero (The More I Love You)Rene & Rene | 26 | Chart history → |
| 15 | Going Up The CountryCanned Heat | 20 | Chart history → |
| 16 | Abraham, Martin And JohnDion | 6 | Chart history → |
| 17 | Crimson And CloverTommy James And The Shondells | 28 | Chart history → |
| 18 | Son-Of-A Preacher ManDusty Springfield | 21 | Chart history → |
| 19 | Bring It On Home To MeEddie Floyd | 17 | Chart history → |
| 20 | See SawAretha Franklin | 14 | Chart history → |
| 21 | Papa's Got A Brand New BagOtis Redding | 24 | Chart history → |
| 22 | Both Sides NowJudy Collins | 11 | Chart history → |
| 23 | Hey JudeThe Beatles | 15 | Chart history → |
| 24 | Magic Carpet RideSteppenwolf | 18 | Chart history → |
| 25 | This Is My CountryThe Impressions | 38 | Chart history → |
| 26 | If I Can DreamElvis Presley | 30 | Chart history → |
| 27 | Everyday PeopleSly & The Family Stone | 42 | Chart history → |
| 28 | Hey JudeWilson Pickett | 43 | Chart history → |
| 29 | Can I Change My MindTyrone Davis | 66 | Chart history → |
| 30 | Scarborough FairSergio Mendes & Brasil '66 | 27 | Chart history → |
| 31 | My SongAretha Franklin | 36 | Chart history → |
| 32 | A Ray Of HopeThe Rascals | 32 | Chart history → |
| 33 | Stand By Your ManTammy Wynette | 34 | Chart history → |
| 34 | Hang 'Em HighBooker T. & The MG's | 40 | Chart history → |
| 35 | There's Gonna Be A ShowdownArchie Bell & The Drells | 49 | Chart history → |
| 36 | Chewy ChewyOhio Express | 19 | Chart history → |
| 37 | Touch MeThe Doors | 72 | Chart history → |
| 38 | Worst That Could HappenBrooklyn Bridge | 53 | Chart history → |
| 39 | Baby Let's WaitThe Royal Guardsmen | 48 | Chart history → |
| 40 | I Started A JokeBee Gees | 41 | Chart history → |
| 41 | Battle Hymn Of The RepublicAndy Williams with the St. Charles Borromeo Choir | 33 | Chart history → |
| 42 | Bella LindaThe Grass Roots | 46 | Chart history → |
| 43 | Are You HappyJerry Butler | 57 | Chart history → |
| 44 | Ready Or Not Here I Come (Can't Hide From Love)The Delfonics | 50 | Chart history → |
| 45 | Little ArrowsLeapy Lee | 22 | Chart history → |
| 46 | My Favorite ThingsHerb Alpert & The Tijuana Brass | 47 | Chart history → |
| 47 | I've Gotta Be MeSammy Davis Jr. | 74 | Chart history → |
| 48 | MalindaBobby Taylor & The Vancouvers | 51 | Chart history → |
| 49 | PeopleThe Tymes | 39 | Chart history → |
| 50 | I Can't Turn You LooseThe Chambers Brothers | 37 | Chart history → |
| 51 | The Beginning Of My EndThe Unifics | 71 | Chart history → |
| 52 | Put Your Head On My ShoulderThe Lettermen | 44 | Chart history → |
| 53 | Baby, Baby Don't CrySmokey Robinson & The Miracles | — | Chart history → |
| 54 | California Dreamin'Bobby Womack | 69 | Chart history → |
| 55 | The Girl Most LikelyJeannie C. Riley | 55 | Chart history → |
| 56 | Crosstown TrafficThe Jimi Hendrix Experience | 56 | Chart history → |
| 57 | California SoulThe 5th Dimension | 62 | Chart history → |
| 58 | Rockin' In The Same Old BoatBobby Bland | 60 | Chart history → |
| 59 | Soul Sister, Brown SugarSam & Dave | 70 | Chart history → |
| 60 | Daddy Sang BassJohnny Cash | 64 | Chart history → |
| 61 | Bluebirds Over The MountainThe Beach Boys | 61 | Chart history → |
| 62 | Shame, ShameMagic Lanterns | 29 | Chart history → |
| 63 | Isn't It Lonely TogetherO.C. Smith | 63 | Chart history → |
| 64 | I Put A Spell On YouCreedence Clearwater Revival | 58 | Chart history → |
| 65 | Ramblin' Gamblin' ManBob Seger System | 75 | Chart history → |
| 66 | Does Anybody Know I'm HereThe Dells | 94 | Chart history → |
| 67 | Just Ain't No LoveBarbara Acklin | 68 | Chart history → |
| 68 | A Minute Of Your TimeTom Jones | 73 | Chart history → |
| 69 | American BoysPetula Clark | 59 | Chart history → |
| 70 | Season Of The Witch, Pt. 1Vanilla Fudge | 65 | Chart history → |
| 71 | White HousesEric Burdon & The Animals | 67 | Chart history → |
| 72 | You Got SoulJohnny Nash | 81 | Chart history → |
| 73 | Rainbow RideAndy Kim | 84 | Chart history → |
| 74 | Condition RedThe Goodees | 97 | Chart history → |
| 75 | Not On The OutsideThe Moments | 85 | Chart history → |
| 76 | Chitty Chitty Bang BangPaul Mauriat | 78 | Chart history → |
| 77 | Electric StoriesThe 4 Seasons Featuring the "Sound of Frankie Valli" | 83 | Chart history → |
| 78 | Feelin' So Good (S.k.o.o.b.y-D.o.o)The Archies | 88 | Chart history → |
| 79 | This Magic MomentJay & The Americans | 90 | Chart history → |
| 80 | VanceRoger Miller | 80 | Chart history → |
| 81 | I Forgot To Be Your LoverWilliam Bell | — | Chart history → |
| 82 | Rain In My HeartFrank Sinatra | — | Chart history → |
| 83 | Shout! - Part 1Chambers Brothers | 96 | Chart history → |
| 84 | Build Me Up ButtercupThe Foundations | — | Chart history → |
| 85 | Sweet Cream Ladies, Forward MarchThe Box Tops | 89 | Chart history → |
| 86 | Tit For Tat (Ain't No Taking Back)James Brown | 86 | Chart history → |
| 87 | KayJohn Wesley Ryles, I | 87 | Chart history → |
| 88 | Ob-La-Di, Ob-La-DaArthur Conley | — | Chart history → |
| 89 | She's A LadyJohn Sebastian | — | Chart history → |
| 90 | You Showed MeThe Turtles | — | Chart history → |
| 91 | EloiseBarry Ryan | 92 | Chart history → |
| 92 | If It Wasn't For Bad LuckRay Charles & Jimmy Lewis | — | Chart history → |
| 93 | You've Got The PowerThe Esquires | 93 | Chart history → |
| 94 | Looking BackJoe Simon | — | Chart history → |
| 95 | The Thought Of Loving YouThe Crystal Mansion | 95 | Chart history → |
| 96 | Things I'd Like To SayNew Colony Six | 100 | Chart history → |
| 97 | I Can't Help It (If I'm Still In Love With You)Al Martino | 99 | Chart history → |
| 98 | I'm Into Lookin' For Someone To Love MeBobby Vee | 98 | Chart history → |
| 99 | Ain't Got No; I Got LifeNina Simone | — | Chart history → |
| 100 | Goodnight My LovePaul Anka | — | Chart history → |