| 1 | I Heard It Through The GrapevineMarvin Gaye | 1 | Chart history → |
| 2 | I'm Gonna Make You Love MeDiana Ross And The Supremes & The Temptations | 2 | Chart history → |
| 3 | Soulful StrutYoung-Holt Unlimited | 4 | Chart history → |
| 4 | Crimson And CloverTommy James And The Shondells | 8 | Chart history → |
| 5 | Hooked On A FeelingB.J. Thomas | 5 | Chart history → |
| 6 | Wichita LinemanGlen Campbell | 3 | Chart history → |
| 7 | For Once In My LifeStevie Wonder | 7 | Chart history → |
| 8 | Touch MeThe Doors | 18 | Chart history → |
| 9 | Worst That Could HappenBrooklyn Bridge | 23 | Chart history → |
| 10 | Son-Of-A Preacher ManDusty Springfield | 13 | Chart history → |
| 11 | CinnamonDerek | 11 | Chart history → |
| 12 | Going Up The CountryCanned Heat | 12 | Chart history → |
| 13 | Cloud NineThe Temptations | 6 | Chart history → |
| 14 | Lo Mucho Que Te Quiero (The More I Love You)Rene & Rene | 14 | Chart history → |
| 15 | Everyday PeopleSly & The Family Stone | 26 | Chart history → |
| 16 | I Started A JokeBee Gees | 19 | Chart history → |
| 17 | If I Can DreamElvis Presley | 17 | Chart history → |
| 18 | Love ChildDiana Ross & The Supremes | 9 | Chart history → |
| 19 | I Love How You Love MeBobby Vinton | 10 | Chart history → |
| 20 | StormyClassics IV Featuring Dennis Yost | 15 | Chart history → |
| 21 | Who's Making LoveJohnnie Taylor | 20 | Chart history → |
| 22 | Abraham, Martin And JohnDion | 16 | Chart history → |
| 23 | Too Weak To FightClarence Carter | 21 | Chart history → |
| 24 | Stand By Your ManTammy Wynette | 33 | Chart history → |
| 25 | Can I Change My MindTyrone Davis | 28 | Chart history → |
| 26 | Hey JudeWilson Pickett | 27 | Chart history → |
| 27 | Hang 'Em HighBooker T. & The MG's | 31 | Chart history → |
| 28 | Bella LindaThe Grass Roots | 38 | Chart history → |
| 29 | California SoulThe 5th Dimension | 34 | Chart history → |
| 30 | This Is My CountryThe Impressions | 25 | Chart history → |
| 31 | Build Me Up ButtercupThe Foundations | 48 | Chart history → |
| 32 | Magic Carpet RideSteppenwolf | 29 | Chart history → |
| 33 | Both Sides NowJudy Collins | 22 | Chart history → |
| 34 | There's Gonna Be A ShowdownArchie Bell & The Drells | 35 | Chart history → |
| 35 | A Ray Of HopeThe Rascals | 24 | Chart history → |
| 36 | Baby Let's WaitThe Royal Guardsmen | 39 | Chart history → |
| 37 | I've Gotta Be MeSammy Davis Jr. | 46 | Chart history → |
| 38 | Hey JudeThe Beatles | 30 | Chart history → |
| 39 | The Beginning Of My EndThe Unifics | 51 | Chart history → |
| 40 | Are You HappyJerry Butler | 42 | Chart history → |
| 41 | Ready Or Not Here I Come (Can't Hide From Love)The Delfonics | 43 | Chart history → |
| 42 | Baby, Baby Don't CrySmokey Robinson & The Miracles | 47 | Chart history → |
| 43 | This Magic MomentJay & The Americans | 65 | Chart history → |
| 44 | Papa's Got A Brand New BagOtis Redding | 37 | Chart history → |
| 45 | California Dreamin'Bobby Womack | 52 | Chart history → |
| 46 | You Showed MeThe Turtles | 72 | Chart history → |
| 47 | Goodnight My LovePaul Anka | 83 | Chart history → |
| 48 | Ramblin' Gamblin' ManBob Seger System | 54 | Chart history → |
| 49 | Does Anybody Know I'm HereThe Dells | 64 | Chart history → |
| 50 | Rainbow RideAndy Kim | 60 | Chart history → |
| 51 | Ob-La-Di, Ob-La-DaArthur Conley | 56 | Chart history → |
| 52 | Soul Sister, Brown SugarSam & Dave | 58 | Chart history → |
| 53 | Daddy Sang BassJohnny Cash | 59 | Chart history → |
| 54 | My Favorite ThingsHerb Alpert & The Tijuana Brass | 45 | Chart history → |
| 55 | A Minute Of Your TimeTom Jones | 55 | Chart history → |
| 56 | Crosstown TrafficThe Jimi Hendrix Experience | 53 | Chart history → |
| 57 | Condition RedThe Goodees | 74 | Chart history → |
| 58 | Things I'd Like To SayNew Colony Six | 82 | Chart history → |
| 59 | You Got SoulJohnny Nash | 70 | Chart history → |
| 60 | Not On The OutsideThe Moments | 75 | Chart history → |
| 61 | Feelin' So Good (S.k.o.o.b.y-D.o.o)The Archies | 63 | Chart history → |
| 62 | Games People PlayJoe South | 91 | Chart history → |
| 63 | Bluebirds Over The MountainThe Beach Boys | 62 | Chart history → |
| 64 | Sweet Cream Ladies, Forward MarchThe Box Tops | 73 | Chart history → |
| 65 | Electric StoriesThe 4 Seasons Featuring the "Sound of Frankie Valli" | 76 | Chart history → |
| 66 | Rain In My HeartFrank Sinatra | 81 | Chart history → |
| 67 | Take Care Of Your HomeworkJohnnie Taylor | — | Chart history → |
| 68 | Isn't It Lonely TogetherO.C. Smith | 68 | Chart history → |
| 69 | I Forgot To Be Your LoverWilliam Bell | 78 | Chart history → |
| 70 | Rockin' In The Same Old BoatBobby Bland | 66 | Chart history → |
| 71 | But You Know I Love YouThe First Edition | — | Chart history → |
| 72 | MalindaBobby Taylor & The Vancouvers | 57 | Chart history → |
| 73 | Looking BackJoe Simon | 94 | Chart history → |
| 74 | I Got A Line On YouSpirit | — | Chart history → |
| 75 | TragedyBrian Hyland | 98 | Chart history → |
| 76 | There'll Come A TimeBetty Everett | — | Chart history → |
| 77 | Home CookinJr. Walker & The All Stars | — | Chart history → |
| 78 | He Called Me BabyElla Washington | — | Chart history → |
| 79 | RiotHugh Masekela | 97 | Chart history → |
| 80 | Almost PersuadedEtta James | — | Chart history → |
| 81 | If It Wasn't For Bad LuckRay Charles & Jimmy Lewis | 90 | Chart history → |
| 82 | Getting The CornersThe T.S.U. Toronadoes | — | Chart history → |
| 83 | KayJohn Wesley Ryles, I | 89 | Chart history → |
| 84 | The Thought Of Loving YouThe Crystal Mansion | 84 | Chart history → |
| 85 | She's A LadyJohn Sebastian | 85 | Chart history → |
| 86 | EloiseBarry Ryan | 86 | Chart history → |
| 87 | Bubble Gum MusicRock & Roll Double Bubble | — | Chart history → |
| 88 | Poor Side Of TownAl Wilson | — | Chart history → |
| 89 | May IBill Deal & The Rhondels | — | Chart history → |
| 90 | The Grooviest Girl In The WorldThe Fun And Games | — | Chart history → |
| 91 | Shout! - Part 1Chambers Brothers | 92 | Chart history → |
| 92 | You've Got The PowerThe Esquires | 93 | Chart history → |
| 93 | Kum Ba YahTommy Leonetti | — | Chart history → |
| 94 | I'm Gonna Hold On Long As I CanThe Marvelettes | — | Chart history → |
| 95 | Ain't Got No; I Got LifeNina Simone | 96 | Chart history → |
| 96 | Will You Be Staying After SundayThe Peppermint Rainbow | — | Chart history → |
| 97 | This Old Heart Of Mine (Is Weak For You)Tammi Terrell | — | Chart history → |
| 98 | Fox On The RunManfred Mann | — | Chart history → |
| 99 | MendocinoSir Douglas Quintet | — | Chart history → |
| 100 | That's Your BabyJoe Tex | — | Chart history → |