| 1 | I Heard It Through The GrapevineMarvin Gaye | 1 | Chart history → |
| 2 | Crimson And CloverTommy James And The Shondells | 4 | Chart history → |
| 3 | I'm Gonna Make You Love MeDiana Ross And The Supremes & The Temptations | 2 | Chart history → |
| 4 | Soulful StrutYoung-Holt Unlimited | 3 | Chart history → |
| 5 | Everyday PeopleSly & The Family Stone | 15 | Chart history → |
| 6 | Hooked On A FeelingB.J. Thomas | 5 | Chart history → |
| 7 | Touch MeThe Doors | 8 | Chart history → |
| 8 | Worst That Could HappenBrooklyn Bridge | 9 | Chart history → |
| 9 | I Started A JokeBee Gees | 16 | Chart history → |
| 10 | Son-Of-A Preacher ManDusty Springfield | 10 | Chart history → |
| 11 | Going Up The CountryCanned Heat | 12 | Chart history → |
| 12 | Can I Change My MindTyrone Davis | 25 | Chart history → |
| 13 | Wichita LinemanGlen Campbell | 6 | Chart history → |
| 14 | For Once In My LifeStevie Wonder | 7 | Chart history → |
| 15 | Hang 'Em HighBooker T. & The MG's | 27 | Chart history → |
| 16 | If I Can DreamElvis Presley | 17 | Chart history → |
| 17 | Cloud NineThe Temptations | 13 | Chart history → |
| 18 | CinnamonDerek | 11 | Chart history → |
| 19 | Love ChildDiana Ross & The Supremes | 18 | Chart history → |
| 20 | I Love How You Love MeBobby Vinton | 19 | Chart history → |
| 21 | There's Gonna Be A ShowdownArchie Bell & The Drells | 34 | Chart history → |
| 22 | Stand By Your ManTammy Wynette | 24 | Chart history → |
| 23 | Too Weak To FightClarence Carter | 23 | Chart history → |
| 24 | Lo Mucho Que Te Quiero (The More I Love You)Rene & Rene | 14 | Chart history → |
| 25 | Hey JudeWilson Pickett | 26 | Chart history → |
| 26 | StormyClassics IV Featuring Dennis Yost | 20 | Chart history → |
| 27 | Who's Making LoveJohnnie Taylor | 21 | Chart history → |
| 28 | Build Me Up ButtercupThe Foundations | 31 | Chart history → |
| 29 | California SoulThe 5th Dimension | 29 | Chart history → |
| 30 | This Is My CountryThe Impressions | 30 | Chart history → |
| 31 | Baby, Baby Don't CrySmokey Robinson & The Miracles | 42 | Chart history → |
| 32 | I've Gotta Be MeSammy Davis Jr. | 37 | Chart history → |
| 33 | Ramblin' Gamblin' ManBob Seger System | 48 | Chart history → |
| 34 | You Showed MeThe Turtles | 46 | Chart history → |
| 35 | Ready Or Not Here I Come (Can't Hide From Love)The Delfonics | 41 | Chart history → |
| 36 | Baby Let's WaitThe Royal Guardsmen | 36 | Chart history → |
| 37 | This Magic MomentJay & The Americans | 43 | Chart history → |
| 38 | The Beginning Of My EndThe Unifics | 39 | Chart history → |
| 39 | Are You HappyJerry Butler | 40 | Chart history → |
| 40 | Take Care Of Your HomeworkJohnnie Taylor | 67 | Chart history → |
| 41 | Bella LindaThe Grass Roots | 28 | Chart history → |
| 42 | Abraham, Martin And JohnDion | 22 | Chart history → |
| 43 | California Dreamin'Bobby Womack | 45 | Chart history → |
| 44 | Papa's Got A Brand New BagOtis Redding | 44 | Chart history → |
| 45 | Goodnight My LovePaul Anka | 47 | Chart history → |
| 46 | A Ray Of HopeThe Rascals | 35 | Chart history → |
| 47 | I'm Livin' In ShameDiana Ross & The Supremes | — | Chart history → |
| 48 | Does Anybody Know I'm HereThe Dells | 49 | Chart history → |
| 49 | Rainbow RideAndy Kim | 50 | Chart history → |
| 50 | Soul Sister, Brown SugarSam & Dave | 52 | Chart history → |
| 51 | Ob-La-Di, Ob-La-DaArthur Conley | 51 | Chart history → |
| 52 | Games People PlayJoe South | 62 | Chart history → |
| 53 | Daddy Sang BassJohnny Cash | 53 | Chart history → |
| 54 | A Minute Of Your TimeTom Jones | 55 | Chart history → |
| 55 | Condition RedThe Goodees | 57 | Chart history → |
| 56 | Things I'd Like To SayNew Colony Six | 58 | Chart history → |
| 57 | Not On The OutsideThe Moments | 60 | Chart history → |
| 58 | You Got SoulJohnny Nash | 59 | Chart history → |
| 59 | Feelin' So Good (S.k.o.o.b.y-D.o.o)The Archies | 61 | Chart history → |
| 60 | I Forgot To Be Your LoverWilliam Bell | 69 | Chart history → |
| 61 | Sweet Cream Ladies, Forward MarchThe Box Tops | 64 | Chart history → |
| 62 | Proud MaryCreedence Clearwater Revival | — | Chart history → |
| 63 | Give It Up Or Turnit A LooseJames Brown | — | Chart history → |
| 64 | Electric StoriesThe 4 Seasons Featuring the "Sound of Frankie Valli" | 65 | Chart history → |
| 65 | Rain In My HeartFrank Sinatra | 66 | Chart history → |
| 66 | But You Know I Love YouThe First Edition | 71 | Chart history → |
| 67 | This Old Heart Of Mine (Is Weak For You)Tammi Terrell | 97 | Chart history → |
| 68 | Home CookinJr. Walker & The All Stars | 77 | Chart history → |
| 69 | There'll Come A TimeBetty Everett | 76 | Chart history → |
| 70 | Looking BackJoe Simon | 73 | Chart history → |
| 71 | RiotHugh Masekela | 79 | Chart history → |
| 72 | River Deep-Mountain HighDeep Purple | — | Chart history → |
| 73 | I Got A Line On YouSpirit | 74 | Chart history → |
| 74 | TragedyBrian Hyland | 75 | Chart history → |
| 75 | Poor Side Of TownAl Wilson | 88 | Chart history → |
| 76 | I'm Gonna Hold On Long As I CanThe Marvelettes | 94 | Chart history → |
| 77 | He Called Me BabyElla Washington | 78 | Chart history → |
| 78 | Purple HazeDion | — | Chart history → |
| 79 | Almost PersuadedEtta James | 80 | Chart history → |
| 80 | If It Wasn't For Bad LuckRay Charles & Jimmy Lewis | 81 | Chart history → |
| 81 | Getting The CornersThe T.S.U. Toronadoes | 82 | Chart history → |
| 82 | The Greatest LoveDorsey Burnette | — | Chart history → |
| 83 | KayJohn Wesley Ryles, I | 83 | Chart history → |
| 84 | She's A LadyJohn Sebastian | 85 | Chart history → |
| 85 | Indian Giver1910 Fruitgum Co. | — | Chart history → |
| 86 | The Grooviest Girl In The WorldThe Fun And Games | 90 | Chart history → |
| 87 | Bubble Gum MusicRock & Roll Double Bubble | 87 | Chart history → |
| 88 | That's Your BabyJoe Tex | 100 | Chart history → |
| 89 | May IBill Deal & The Rhondels | 89 | Chart history → |
| 90 | Let It Be MeGlen Campbell & Bobbie Gentry | — | Chart history → |
| 91 | You've Got The PowerThe Esquires | 92 | Chart history → |
| 92 | Kum Ba YahTommy Leonetti | 93 | Chart history → |
| 93 | The Carroll County AccidentPorter Wagoner | — | Chart history → |
| 94 | Ain't Got No; I Got LifeNina Simone | 95 | Chart history → |
| 95 | Will You Be Staying After SundayThe Peppermint Rainbow | 96 | Chart history → |
| 96 | MendocinoSir Douglas Quintet | 99 | Chart history → |
| 97 | Fox On The RunManfred Mann | 98 | Chart history → |
| 98 | Please Don't Desert Me BabyGloria Walker/Chevelles | — | Chart history → |
| 99 | CrossroadsCream | — | Chart history → |
| 100 | Hey! BabyJose Feliciano | — | Chart history → |